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Record W2914186641 · doi:10.1002/cjce.23468

Review of fluid‐solid reaction analysis—Part 2: Single porous reactant solid

2019· article· en· W2914186641 on OpenAlexvenueno aff
Hong Yong Sohn

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2019
Typearticle
Languageen
FieldEnvironmental Science
TopicCoagulation and Flocculation Studies
Canadian institutionsnot available
Fundersnot available
KeywordsPorositySolid solutionSolid surfaceMaterials sciencePorous mediumSolid acidReaction rateSimple (philosophy)Point (geometry)ThermodynamicsChemical engineeringMechanicsChemistryMathematicsPhysicsComposite materialChemical physicsGeometryCatalysisMetallurgyEngineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Part 1of this series covered the reaction of a non‐porous solid.[1] In this Part 2 of the series, we present a review on the reactions involving a porous solid, which is the most widely encountered type of fluid‐solid reactions. The major difference between the reactions of a non‐porous and a porous solid is the fact that in the latter, the fluid reactant can reach the interior of the porous solid through the pores even through a portion that contains unreacted solid reactant. The rate expression for the solid at any point depends on, among others, how the area of reaction interface changes with the conversion of the solid. The governing equations, in general, require numerical solution. In this article we describe an approximate closed‐form solution to this problem that yielded Sohn's law of additive reaction times. The result is simple to apply and has many useful features, especially for the design and modelling of a multi‐particle system.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.003
Threshold uncertainty score0.011

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0030.003
Science and technology studies0.0000.001
Scholarly communication0.0010.003
Open science0.0020.001
Research integrity0.0020.002
Insufficient payload (model declined to judge)0.0030.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.218
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2019
Admission routes1
Has abstractyes

Explore more

Same venueThe Canadian Journal of Chemical EngineeringSame topicCoagulation and Flocculation StudiesFrench-language works237,207