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Record W2914439665 · doi:10.1103/physrevb.99.045135

Suppression of long-range ferromagnetic order in the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Ce</mml:mi><mml:mi>x</mml:mi></mml:msub><mml:msub><mml:mi>La</mml:mi><mml:mrow><mml:mn>1</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi>TiGe</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math> system

2019· article· lv· W2914439665 on OpenAlexafffund
Jeong Hun Lee, Anja Rabus, Chris Coutts, Eundeok Mun

Bibliographic record

VenuePhysical review. B./Physical review. B · 2019
Typearticle
Languagelv
FieldPhysics and Astronomy
TopicRare-earth and actinide compounds
Canadian institutionsSimon Fraser University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsCondensed matter physicsElectrical resistivity and conductivityPhysicsFerromagnetismPhase diagramMagnetizationMagnetic susceptibilityOrder (exchange)Materials scienceMagnetic fieldPhase (matter)Quantum mechanics

Abstract

fetched live from OpenAlex

We report specific heat, magnetization, and resistivity measurements on single crystals of ${\mathrm{Ce}}_{x}{\mathrm{La}}_{1\ensuremath{-}x}{\mathrm{TiGe}}_{3}$ systems. When the Ce concentration $x$ is increased, the system changes from a single-ion Kondo system for $x=0.05$ into a ferromagnetic Kondo lattice for $x=1$, where the magnetic part of electrical resistivity reveals a single-ion scaling with $x$. The isoelectric substitution of Ce by La atoms causes a change of the relative strength of competing energy scales of Kondo and RKKY interaction and crystalline electric field (CEF). The substitutions induce the continuous evolution of the Kondo temperature ${T}_{K}$ and the linear variation of ferromagnetic ordering temperature ${T}_{c}$, which are accompanied by a change of the CEF level scheme of the Ce ions. The composition-temperature ($x\text{\ensuremath{-}}T$) phase diagram for ${\mathrm{Ce}}_{x}{\mathrm{La}}_{1\ensuremath{-}x}{\mathrm{TiGe}}_{3}$ is constructed by a combination of magnetization, specific heat, and resistivity measurements. The ferromagnetic ordering temperature is linearly suppressed as $x$ decreases and vanishes near the critical concentration ${x}_{c}=0.1$, but conventional quantum criticality is absent near ${x}_{c}$. The specific heat measurement for $x=0.05$ reveals the power law increase of the electronic specific heat coefficient ${C}_{m}/T\ensuremath{\propto}1/T$ with a large value of $\ensuremath{\sim}3.5$ J/mol ${\mathrm{K}}^{2}$ at $T=0.4\phantom{\rule{0.28em}{0ex}}\mathrm{K}$. The magnetic susceptibility for $x=0.05$ also shows a power law dependence $\ensuremath{\chi}(T)\ensuremath{\propto}1/T$ below 10 K.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.006
metaresearch head score (Gemma)0.004
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Open science, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Science and technology studies, Research integrity, Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.927
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0060.004
Meta-epidemiology (narrow)0.0030.006
Meta-epidemiology (broad)0.0020.008
Bibliometrics0.0010.005
Science and technology studies0.0040.004
Scholarly communication0.0040.004
Open science0.0080.006
Research integrity0.0040.006
Insufficient payload (model declined to judge)0.6820.010

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.268
Teacher spread0.251 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2019
Admission routes2
Has abstractyes

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