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Characterization of Shale Pore Size Distribution by NMR Considering the Influence of Shale Skeleton Signals

2019· article· en· W2950006358 on OpenAlexaff
Jinbu Li, Shuangfang Lu, Chunqing Jiang, Min Wang, Zhuoheng Chen, Guohui Chen, Jijun Li, Shudong Lu

Bibliographic record

VenueEnergy & Fuels · 2019
Typearticle
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsGeological Survey of Canada
FundersMinistry of Science and Technology of the People's Republic of ChinaMinistry of Education of the People's Republic of ChinaMinistry of Human Resources and Social SecurityNational Natural Science Foundation of China
KeywordsOil shaleShale oilKerogenChemistryRelaxometryCarbon-13 NMRNMR spectra databaseProton NMRMineralogyAnalytical Chemistry (journal)Spectral lineGeologyOrganic chemistrySpin echoSource rockMagnetic resonance imaging

Abstract

fetched live from OpenAlex

As a non-destructive method, the proton nuclear magnetic resonance (1H NMR) technique with low echo time (TE, e.g., 0.07 ms) has been increasingly used for characterizing full pore size distribution (PSD) of shales. However, hydrogen contained in some components of the shale skeleton (e.g., kerogen and structural water) also can be detected by NMR in the case of low TE, resulting in a questionable PSD derived directly from the T2 spectra of oil-saturated shale. In this study, eight shale samples with different organic and mineralogical components from the Jiyang Depression, China were investigated with regular NMR, low-temperature nitrogen adsorption (LTNA), NMR cryoporometry (NMRC), and mercury injection capillary pressure (MICP) techniques to propose a corrected NMR approach for characterizing shale PSD by considering the influence of the shale skeleton signals. The NMR relaxation characteristics (e.g., T2 spectra and T1–T2 map) of as-received shale, solvent-extracted and dried shale (EX), and oil-saturated shale (OS) were discussed to reveal the NMR response from the shale skeleton itself at T2 below 1 ms on the T2 spectra. With the new approach, the NMR T2 spectra of oil occurring in the OS shale were first obtained through inversion of the differentiated T2 decay curves between the T2 decay curves of the EX shale and OS shale and were then converted to PSD by combination of LTNA, NMRC, and MICP results. For pores with T2 less than 1 ms, the PSD obtained from NMR T2 spectra of the oil signals only compared well with the results of LTNA and NMRC, with a relative error of less than 15% in pore volume. In contrast, the relative errors of PSD obtained directly from the NMR T2 spectra of oil-saturated shales were up to 134%. It was found that the higher total organic carbon shale contained, the larger errors in the PSD profiles, pore volume, and porosity that were calculated directly from the oil-saturated shale’s NMR T2 spectra. Compared with the traditional NMR methods, the corrected approach can provide a more accurate PSD for shales, especially for those organic-rich ones.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.049
Threshold uncertainty score0.366

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.190
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations40
Published2019
Admission routes1
Has abstractyes

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