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Intrinsic insulating ground state in transition metal dichalcogenide <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi>TiSe</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:math>

2019· article· lv· W2950900286 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenuePhysical Review Materials · 2019
Typearticle
Languagelv
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsCanadian Institute for Advanced ResearchUniversity of British Columbia
FundersAir Force Office of Scientific ResearchWorkforce Development for Teachers and ScientistsDivision of Materials ResearchBasic Energy SciencesNatural Sciences and Engineering Research Council of CanadaOak Ridge Institute for Science and EducationUniversity of TokyoOffice of ScienceCanada First Research Excellence FundCanada Research ChairsCanada Foundation for InnovationCanadian Institute for Advanced ResearchCummings FoundationKillam TrustsGordon and Betty Moore FoundationArgonne National LaboratoryU.S. Department of EnergyNational Science Foundation
KeywordsGround stateElectrical resistivity and conductivityMagnetismTransition metalFermi levelArgonInert gasBar (unit)Inert

Abstract

fetched live from OpenAlex

The transition metal dichalcogenide ${\mathrm{TiSe}}_{2}$ has received significant research attention over the past four decades. Different studies have presented ways to suppress the 200 K charge-density-wave transition, vary low-temperature resistivity by several orders of magnitude, and stabilize magnetism or superconductivity. Here we give the results of a synthesis technique whereby samples were grown in a high-pressure environment with up to 180 bar of argon gas. Above 100 K, properties are nearly unchanged from previous reports, but a distinct hysteretic resistance region begins around 80 K, accompanied by insulating low-temperature behavior. An accompanying decrease in carrier concentration is seen in Hall effect measurements, and photoemission data show a removal of an electron pocket from the Fermi surface in an insulating sample. We conclude that high inert gas pressure synthesis accesses an underlying nonmetallic ground state in a material long speculated to be an excitonic insulator.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Scholarly communication, Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.501
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.1200.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.266
Teacher spread0.244 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it