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Correcting <i>T</i><sub>max</sub> Suppression: A Numerical Model for Removing Adsorbed Heavy Oil and Bitumen from Upper Ordovician Source Rocks, Arctic Canada

2019· article· en· W2951628325 on OpenAlexafffundabout
Zhuoheng Chen, Keith Dewing, Dane P. Synnott, Xiaojun Liu

Bibliographic record

VenueEnergy & Fuels · 2019
Typearticle
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsUniversity of CalgaryGeological Survey of Canada
FundersNatural Resources CanadaCoordenação de Aperfeiçoamento de Pessoal de Nível Superior
KeywordsKerogenSource rockPetroleumAdsorptionMineralogyHydrocarbonPyrolysisGeologySorptionPetroleum geochemistryDissolutionAsphaltAnalytical Chemistry (journal)ChemistryEnvironmental chemistryMaterials scienceOrganic chemistryGeomorphology

Abstract

fetched live from OpenAlex

A Rock-Eval 6 dataset of 66 samples from the Cape Phillips Formation in the Canadian Arctic region was studied to investigate source rock characteristics and petroleum generation potential. Bulk geochemical characteristics and thermal decomposition behavior of the samples indicate an initial generation potential close to 700 mg HC/g TOC and show an unusually low onset T max temperature for petroleum generation. This led to an examination of possible T max suppression due to a large amount of high-molecular-weight heavy oil and bitumen derived from the early breakdown of kerogen in the samples. Application of a numerical method based on kerogen decomposition kinetics allows for the numerical removal of thermal evaporative products of oil and bitumen adsorbed in the sample without requiring additional pyrolysis experiments or solvent extraction treatments of sample replicates. The removal of the adsorbed hydrocarbon from samples increases the T max value up to 17 °C. The estimated petroleum in the sorption phase varies from 1 to about 9 mg HC/g rock, depending on the total organic content (TOC) and maturity, and is the main form of the total oil yield in this area. The corrected T max –HI cross-plot suggests an onset of petroleum generation around 435 °C of T max, consistent with the general consensus for a normal marine source rock in this region. The constructed kinetic model shows a maximum of 75% transformation ratio (TR), and most samples show TR ranging from 10 to 50% in the early oil generation window on Cornwallis Island. This reconstructed source rock thermal decomposition model in a geological time scale indicates the onset of massive petroleum generation at a temperature of 120 °C, and the maximum transformation ratio of 75% corresponds to a temperature of 140 °C over geological time.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.304
Threshold uncertainty score0.611

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.000
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.186
Teacher spread0.180 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2019
Admission routes3
Has abstractyes

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