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Record W2956649489 · doi:10.1021/acsomega.9b01039

Melanin: A Greener Route To Enhance Energy Storage under Solar Light

2019· article· en· W2956649489 on OpenAlexafffund
Ri Xu, Abdelaziz Gouda, Maria Federica Caso, Francesca Soavi, Clara Santato

Bibliographic record

VenueACS Omega · 2019
Typearticle
Languageen
FieldEngineering
TopicElectrochemical sensors and biosensors
Canadian institutionsPolytechnique Montréal
FundersNatural Sciences and Engineering Research Council of CanadaFonds Québécois de la Recherche sur la Nature et les TechnologiesMinistère des relations internationales et de la Francophonie
KeywordsSupercapacitorCapacitanceEnergy storageMaterials scienceRenewable energyOptoelectronicsFaraday efficiencyEnergy conversion efficiencyEnergy transformationElectrodeSolar energyElectrolyteNanotechnologyChemistryPower (physics)PhysicsElectrical engineeringEngineering

Abstract

fetched live from OpenAlex

The development of technologies integrating solar energy conversion and energy storage functions is critical for limiting the anthropogenic effects on climate change and preventing possible energy shortages related to the increase of the world population. In our work, we explored the possibility to integrate the conversion and storage functions within the same multifunctional biosourced material. We identified the redox-active, quinone-based, melanin pigment, featuring a broadband absorption in the UV-vis region, as the ideal candidate for such an exploration. Electrodes of melanin on carbon paper were investigated for their morphological, optical, and voltammetric characteristics prior to being assembled into symmetric supercapacitors operating in aqueous electrolytes. We observed that, under solar light, the capacity and capacitance of melanin electrodes significantly increase with respect to the dark conditions (by 22 and 39%, respectively). Once in a supercapacitor configuration, besides featuring a Coulombic efficiency close to 100% after 5000 cycles, the capacitance and capacity of the electrodes, rated by the initial values, improve after prolonged illumination, as it is the case for the energy and power density.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.192
Teacher spread0.188 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations80
Published2019
Admission routes2
Has abstractyes

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