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Record W2964713071 · doi:10.1103/physrevb.100.075143

Spin-orbit excitons in CoO

2019· article· en· W2964713071 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenuePhysical review. B./Physical review. B · 2019
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAdvanced Condensed Matter Physics
Canadian institutionsNational Research Council Canada
FundersEngineering and Physical Sciences Research CouncilUniversity of California, Santa BarbaraOffice of ScienceScience and Technology Facilities CouncilUniversity of EdinburghEuropean Research CouncilRoyal Society of ChemistryRoyal SocietyBasic Energy SciencesCarnegie Trust for the Universities of ScotlandU.S. Department of Energy
KeywordsPhysicsAntiferromagnetismCondensed matter physicsMott insulatorSpin (aerodynamics)Lattice (music)Atomic physics

Abstract

fetched live from OpenAlex

CoO has an odd number of electrons in its unit cell, and therefore is expected to be metallic. Yet, CoO is strongly insulating owing to significant electronic correlations, thus classifying it as a Mott insulator. We investigate the magnetic fluctuations in CoO using neutron spectroscopy. The strong and spatially far-reaching exchange constants reported recently [P. M. Sarte et al., Phys. Rev. B 98, 024415 (2018)], combined with the single-ion spin-orbit coupling of similar magnitude [R. A. Cowley et al., Phys. Rev. B 88, 205117 (2013)] results in significant mixing between $j{}_{\mathrm{eff}}$ spin-orbit levels in the low-temperature magnetically ordered phase. The high degree of entanglement, combined with the structural domains originating from the Jahn-Teller structural distortion at $\ensuremath{\sim}300\phantom{\rule{0.28em}{0ex}}\mathrm{K}$, make the magnetic excitation spectrum highly structured in both energy and momentum. We extend previous theoretical work on ${\mathrm{PrTl}}_{3}$ [W. J. L. Buyers et al., Phys. Rev. B 11, 266 (1975)] to construct a mean-field and multilevel spin-orbit exciton model employing the aforementioned spin exchange and spin-orbit coupling parameters for coupled ${\mathrm{Co}}^{2+}$ ions lying on a rocksalt lattice. This parametrization, based on a tetragonally distorted type-II antiferromagnetic unit cell, captures both the sharp low-energy excitations at the magnetic zone center, and the energy broadened peaks at the zone boundary. However, the model fails to describe the momentum dependence of the excitations at high-energy transfers, where the neutron response decays faster with momentum than the ${\mathrm{Co}}^{2+}$ form factor. We discuss such a failure in terms of a possible breakdown of localized spin-orbit excitons at high-energy transfers.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: Theoretical or conceptual
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.153
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0030.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.009

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.369
Teacher spread0.358 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it