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Record W2965197627 · doi:10.1002/etc.4557

The Effect of Major Ions and Dissolved Organic Matter on Complexation and Toxicity of Dissolved Thallium to <i>Daphnia magna</i>

2019· article· en· W2965197627 on OpenAlexaff
Andrew Nagel, Chad W. Cuss, Greg G. Goss, William Shotyk, Chris N. Glover

Bibliographic record

VenueEnvironmental Toxicology and Chemistry · 2019
Typearticle
Languageen
FieldEnvironmental Science
TopicThallium and Germanium Studies
Canadian institutionsAthabasca UniversityUniversity of Alberta
Fundersnot available
KeywordsDaphnia magnaEnvironmental chemistryChemistryThalliumFractionationToxicityGenetic algorithmBiogeochemical cycleDissolved organic carbonMetalMetal ions in aqueous solutionInorganic chemistryChromatographyEcologyBiologyOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Thallium (Tl) is a trace element associated with base metal mining and processing, but little is known regarding how its toxicity is influenced by water chemistry. In the present study, the 48-h median lethal concentration (LC50) of Tl to Daphnia magna was determined in a standard laboratory water, and toxicity was reassessed under conditions of varying cation (Ca2+, K+, Na+), anion (Cl–, HCO–3), and dissolved organic matter (DOM) concentrations. The calculated 48-h LC50 of 1.86 mg Tl/L was consistent with previous work on Tl toxicity to D. magna. At the 48-h LC50 concentration, changes in water chemistry had no statistically significant effect on mortality, although there was a trend toward lower Tl toxicity with elevated water K+. Test waters containing 10 mM CaCl2 did not support control survival. The measurement of Tl complexation with DOM using asymmetric flow field flow fractionation confirmed the outcomes of biogeochemical speciation modeling: Tl speciation was relatively unaffected by water chemistry, and the majority of Tl remained in the ionic form across all treatments. These data indicate that Tl toxicity is largely independent of speciation, a property that will greatly simplify risk assessments for this metal in freshwaters. Environ Toxicol Chem 2019;38:2472–2479. © 2019 SETAC

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score0.014

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.184
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2019
Admission routes1
Has abstractyes

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