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Record W2967762692 · doi:10.1002/aenm.201900889

Rational Design of Novel Catalysts with Atomic Layer Deposition for the Reduction of Carbon Dioxide

2019· article· en· W2967762692 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Energy Materials · 2019
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsInstitut National de la Recherche Scientifique
FundersFonds de recherche du Québec – Nature et technologiesNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of ChinaInstitut national de la recherche scientifique
KeywordsAtomic layer depositionCatalysisMaterials scienceNanomaterialsNanotechnologySelective catalytic reductionElectrochemical reduction of carbon dioxideGreenhouse gasCombustionCarbon fibersReduction (mathematics)Deposition (geology)Layer (electronics)Chemical engineeringCarbon monoxideChemistryOrganic chemistryComposite numberEngineering

Abstract

fetched live from OpenAlex

Abstract Carbon dioxide (CO 2 ) is one of the end products of fuel combustion and the major component of the greenhouse gases. The reduction of atmospheric CO 2 not only decreases environmental pollution but also produces value‐added chemicals, solving energy and environment issues simultaneously. One significant challenge is the low conversion efficiency of CO 2 reduction due to the inertness of the CO 2 molecule. The design of the catalyst nanomaterials with the high selectivity, stability, and the activation capabilities for the conversion of CO 2 is needed. Atomic layer deposition (ALD), capable of constructing catalysts with atomic‐level precision in a highly controllable manner, is a promising technique to address the key problems in CO 2 reduction. This review explores the application of ALD in CO 2 reduction, emphasizing the designs of the efficient catalyst nanomaterials fabricated by the ALD technique and their applications in CO 2 reduction and capture. The significance of the ALD catalysts with the fine structures is highlighted to obtain a better understanding of the catalytic performance–aimed benefits as well as an outlook on the ALD‐designed catalysts for the reduction of CO 2 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.094
Threshold uncertainty score0.473

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.246
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it