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Record W2979860422 · doi:10.5194/acp-20-2277-2020

Ammonia measurements from space with the Cross-track Infrared Sounder: characteristics and applications

2020· article· en· W2979860422 on OpenAlexafffundabout
Mark W. Shephard, Enrico Dammers, Karen Cady‐Pereira, Shailesh Kumar Kharol, Jesse Thompson, Yonatan Gainariu-Matz, Junhua Zhang, C. A. McLinden, Andrew Kovachik, Michael D. Moran, Shabtai Bittman, Christopher E. Sioris, Debora Griffin, M. J. Alvarado, C. R. Lonsdale, Verica Savic-Jovcic, Qiong Zheng

Bibliographic record

VenueAtmospheric chemistry and physics · 2020
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsAgriculture and Agri-Food CanadaUniversity of WaterlooPublic Health OntarioUniversity of TorontoEnvironment and Climate Change Canada
FundersClimate Program OfficeNuclear Safety and Security CommissionNational Oceanic and Atmospheric AdministrationGovernment of AlbertaEnvironment and Climate Change CanadaNational Aeronautics and Space Administration
KeywordsEnvironmental scienceAmmoniaSatelliteAtmospheric sciencesLatitudeReactive nitrogenAir quality indexMeteorologyClimatologyNitrogenGeographyChemistryPhysics

Abstract

fetched live from OpenAlex

Abstract. Despite its clear importance, the monitoring of atmospheric ammonia, including its sources, sinks, and links to the greater nitrogen cycle, remains limited. Satellite data are helping to fill the gap in monitoring from sporadic conventional ground- and aircraft-based observations to better inform policymakers and assess the impact of any ammonia-related policies. Presented is a description and survey that demonstrate the capabilities of the Cross-track Infrared Sounder (CrIS) ammonia product for monitoring, air quality forecast model evaluation, dry deposition estimates, and emission estimates from an agricultural hotspot. For model evaluation, while there is a general agreement in the spatial allocation of known major agricultural ammonia hotspots across North America, the satellite observations show some high-latitude regions during peak forest fire activity often have ammonia concentrations approaching those in agricultural hotspots. The CrIS annual ammonia dry depositions in Canada (excluding the territories) and the US have average and annual variability values of ∼0.8±0.08 and ∼1.23±0.09 Tg N yr−1, respectively. These satellite-derived dry depositions of reactive nitrogen from NH3 with NO2 show an annual ratio of NH3 compared to their sum (NH3+NO2) of ∼82 % and ∼55 % in Canada and the US, respectively. Furthermore, we show the use of CrIS satellite observations to estimate annual and seasonal emissions near Lethbridge, Alberta, Canada, a region dominated by high-emission concentrated animal feeding operations (CAFOs); the satellite annual emission estimate of 37.1±6.3 kt yr−1 is at least double the value reported in current bottom-up emission inventories for this region.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.174
Threshold uncertainty score0.804

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.204
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations105
Published2020
Admission routes3
Has abstractyes

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