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Record W2996514253 · doi:10.3390/catal9121045

Passive Solar Photocatalytic Treatment of Emerging Contaminants in Water: A Field Study

2019· article· en· W2996514253 on OpenAlex
Gisoo Heydari, Cooper H. Langford, Gopal Achari

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueCatalysts · 2019
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsUniversity of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaMitacs
KeywordsPhotocatalysisDegradation (telecommunications)ChemistryAcetic acidEnvironmental chemistryBenzoic acidContaminationSulfolaneAqueous solutionNuclear chemistryOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

Global economic shifts towards utilization of solar energy provides opportunities for photocatalytic technologies that can harness this abundant source of energy for treatment of organic contaminants. The majority of studies in this area have been performed under artificial light, whereas in this paper, the efficacy of passive photocatalysis was studied under sunlight. Buoyant titanium dioxide (TiO2) coated glass spheres were used to treat 2, 4-dichlorophenoxy acetic acid (2, 4-D), methyl chlorophenoxy propionic acid (MCPP), and 3, 6-Dichloro-2-methoxy benzoic acid (Dicamba) in Killex®, a commercially available herbicide. Furthermore, photocatalytic degradation of sulfolane and a typical naphthenic acid (cyclopentane carboxylic acid—CPA) were also tested under ambient conditions. The results showed 99.8% degradation of 2, 4-D, 100% degradation of both MCPP and Dicamba in Killex® solution, and 97.4% degradation of sulfolane by capturing 3.18 MJ/m2 solar energy. Total organic carbon (TOC) was decreased by 88% and 64% in both solutions, respectively. TOC of the aqueous solution containing 20 ppm CPA was also decreased by 78.4% with 7.8 MJ/m2 energy. Despite the slow kinetics and the temporal variations of sunlight in northern latitudes, the results indicated that passive photocatalysis is a promising approach for treatment of contaminants under ambient conditions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.431
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.249
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it