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Record W2997546427 · doi:10.1002/9780470682531.pat0974

Photochemical Transformations Involving Organoboron

2019· other· en· W2997546427 on OpenAlexaff
Soren K. Mellerup, Suning Wang

Bibliographic record

Venuenot available
Typeother
Languageen
FieldMaterials Science
TopicPhotochromic and Fluorescence Chemistry
Canadian institutionsQueen's University
Fundersnot available
KeywordsChemistryIsostructuralPhotochromismPhotochemistryBoronMoleculeSynthonElectron deficiencyComputational chemistryCrystallographyOrganic chemistryCrystal structure

Abstract

fetched live from OpenAlex

Abstract Boron gets its name from the term borax, the mineral from which it was originally isolated, by analogy with carbon due to their chemical similarities. Unlike its neighbor on the periodic table, however, boron only possesses enough valence electrons to form three covalent bonds. This means that organoboron compounds are inherently electron deficient and typically adopt a trigonal‐planar (sp 2 ‐hybridized) geometry with the empty p z orbital of boron lying orthogonal to the bonding plane. In this form, boron is isoelectronic and isostructural with a positively charged carbocation, which gives rise to many of the applications often associated with trivalent organoboranes (e.g., organic synthons and electron‐transport materials). Coordinatively saturating these systems with anionic or neutral Lewis bases yields tetrahedral, four‐coordinated boron compounds with a formal negative charge. This new bonding arrangement significantly alters the orbital composition of the resulting molecules, imparting new features such as intense charge transfer (CT) luminescence and, in some cases, unique photochemical reactivities such as photochromism or photoelimination. This chapter will document recent progress in photochemical transformation based on organoboron compounds. A brief overview of concepts related to photophysical and photochemical processes will be presented, followed by an introduction to photochromic systems and a comprehensive review of organoboron photochemistry. Several recently discovered classes of photoresponsive organoboron molecules and their potential applications will be presented.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.282
Threshold uncertainty score0.995

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0560.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.221
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2019
Admission routes1
Has abstractyes

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