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Record W3000683664 · doi:10.3390/atmos11010073

Comparison of Atmospheric Mercury Speciation at a Coastal and an Urban Site in Southeastern Texas, USA

2020· article· en· W3000683664 on OpenAlexaff
Travis Griggs, Lei Liu, R. W. Talbot, Azucena Torres, Xin Lan

Bibliographic record

VenueAtmosphere · 2020
Typearticle
Languageen
FieldEnvironmental Science
TopicMercury impact and mitigation studies
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsSunriseMercury (programming language)Mixing ratioEnvironmental scienceParticulatesSouthern HemisphereNorthern HemisphereAtmospheric sciencesOceanographyEnvironmental chemistryClimatologyGeologyChemistry

Abstract

fetched live from OpenAlex

Sixteen months of continuous measurements and the analysis of atmospheric mercury (gaseous elemental mercury GEM, gaseous oxidized mercury GOM, and particulate bound mercury PBM) under urban and coastal settings were conducted in Southeastern Texas. At the urban site, the GEM mean mixing ratio was 185 ppqv, 5%–10% higher than the Northern Hemisphere GEM background level. GOM and PBM mixing ratios were as much as six times higher than their background level. The coastal site GEM mean mixing ratio was 165 ppqv, higher than other coastal sites located in the Northern Hemisphere. GOM and PBM mean mixing ratios at the coastal site were 0.75 ppqv and 0.58 ppqv. The urban site had a higher frequency of high mercury events (>300 ppqv) compared to the coastal site. The diurnal patterns were found for both sites: In the urban environment, GEM accumulated to the maximum mixing ratio just after sunrise and decreased to the minimum mixing ratio in late afternoon. In the coastal environment, GEM decreased at night reaching its minimum mixing ratio before sunrise. The relationship between atmospheric mercury species and meteorological parameters was investigated. An examination of the relationship between atmospheric mercury species and key trace gases was conducted as well, showing that the concurrence of GEM, CO2, CO, CH4, and SO2 maximum mixing ratios was notable and provided evidence they may originate from the same emission source. The coastal site was at times influenced by polluted air from urban Houston and the cleaner Gulf of Mexico marine air at other times.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.277
Teacher spread0.252 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2020
Admission routes1
Has abstractyes

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