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Record W3007996018 · doi:10.6000/1929-5995.2020.09.01

Mono- and Bis- Maleimide Resins in Preimpregnated Fibres

2020· article· en· W3007996018 on OpenAlexvenueno aff
Heinrich Horacek

Bibliographic record

VenueJournal of Research Updates in Polymer Science · 2020
Typearticle
Languageen
FieldMaterials Science
TopicSynthesis and properties of polymers
Canadian institutionsnot available
Fundersnot available
KeywordsMaterials scienceGlass transitionMaleimideDifferential scanning calorimetryCuring (chemistry)MethylenePolymer chemistryAnilineCopolymerPolymerizationPolymerStyreneComposite materialOrganic chemistryChemistry

Abstract

fetched live from OpenAlex

Fibres are preimpregnated by solutions of mono- and bis-maleimides with comonomers. Imides alone polymerize to resins with too low energies of fracture. In the presence of Methylene dianiline or Aniline Diphenylmethylenebismaleimide reacts via Michael addition to equimolar addition products. When fibres are preimpregnated with these addition compounds alone or in combination with flame retardants, B-prepregs are obtained, which after curing show high glass temperatures and sufficient energies of fracture. 2.5 moles of Diphenylmethylene bismaleimide and 1mol Methylene dianiline or 1mole Aniline react to resins with glass temperatures of 350 and 380°C and energies of fracture of 75 and 100J/m2. The resins contain no carcinogen or blood harming free amines. A one pot reaction starting from Methylene dianiline and Maleic anhydride is possible and more economic. As polymerized bismaleimides possess their imide bonds in the side chain, they are strictly spoken no polyimides with imide bonds in the main chain. Diphenylmethylenebismaleimide and styrene as copolymer react to an insoluble crosslinked polymer. Fibres are preimpregnated with equimolar mixtures of 2- Bromophenylmaleimide and styrene. After curing laminates with 285°C glass temperature and sufficient energies of fracture are obtained. The heat resistant resins are charring polymers and display higher Limiting Oxygen Indices, when the heats of combustion are increased. Differential Scanning Calorimetry determines the temperatures and the heats of glass transition, which indicate that the glass temperature is raised, when the enthalpy is increased and the entropy reduced, which is achievable by Diphenylbismaleimide and 2-Bromophenylmaleimide with their large side groups appropriate for intermolecular forces and steric hindrance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.074
GPT teacher head0.357
Teacher spread0.283 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2020
Admission routes1
Has abstractyes

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