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Record W3013242634 · doi:10.1139/cjp-2019-0558

Tailoring electronic and optical properties of LaAlO<sub>3</sub> by Cu inclusion: a DFT study

2020· article· en· W3013242634 on OpenAlexvenueno aff
Muhammad Rizwan, Sadia H. Gul, Tariq Mahmood, M. Shakil‎, Abdul Majid, Muhammad Rafique, A. A. Zafar, Haibo Jin, Chuanbao Cao

Bibliographic record

VenueCanadian Journal of Physics · 2020
Typearticle
Languageen
FieldMaterials Science
TopicElectronic and Structural Properties of Oxides
Canadian institutionsnot available
Fundersnot available
KeywordsPhysicsDopingDensity functional theoryBand gapAbsorption edgeCondensed matter physicsValence (chemistry)Context (archaeology)Electronic structureRefractive indexRedshiftDensity of statesElectronic band structureOptoelectronicsQuantum mechanics

Abstract

fetched live from OpenAlex

First principles calculations in the context of density functional theory (DFT) provides a platform to investigate the material’s properties in a way to explain the physics of solids. Electronic, structural, and optical properties for pure and Cu-doped LaAlO 3 are investigated. The study reveals that the band structure of LaAlO 3 after the inclusion of Cu at the La site is affected significantly. Due to the substitution of Cu, there is a decrease in the band gap from 3.02 eV to 2.95 eV. Furthermore, the partial density of states of LaAlO 3 changes significantly after Cu doping, which has confirmed the doping effect on intrinsic LaAlO 3 . The p and d states play a vital role on top of the valence band. The range in which the top of a valence band lies is from 0 eV to –9 eV having a significant effect and it is because of Cu-d states. The optical properties of both pure and doped systems were analyzed. Redshift was observed as absorption edge shifted from 4.5 eV to 4.0 eV and even the refractive index reduces from 2.25 to 1.0, which means the Cu inclusion significantly play its role to tailor optical properties. Hence Cu-doping affects the properties of LaAlO 3 and makes it a suitable candidate for use in different optical devices.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.200
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations29
Published2020
Admission routes1
Has abstractyes

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Same venueCanadian Journal of PhysicsSame topicElectronic and Structural Properties of OxidesFrench-language works237,207