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Record W3013304191 · doi:10.1002/aic.16977

Quantitative distinction of thermodynamic soluble and miscible states

2020· article· en· W3013304191 on OpenAlexaff
Kaiqiang Zhang, Na Jia, Lirong Liu

Bibliographic record

VenueAIChE Journal · 2020
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsUniversity of Regina
Fundersnot available
KeywordsSolubilityThermodynamicsTernary operationHildebrand solubility parameterChemistryBinary numberWork (physics)Flory–Huggins solution theoryOrganic chemistryMathematicsPhysicsPolymer

Abstract

fetched live from OpenAlex

Abstract Soluble and miscible states are two important thermodynamic states in academic research and practical applications but their quantitative distinctions are still fuzzy. In this study, for the first time, the mathematical formulations of the quantitative criteria for distinguishing the thermodynamic soluble and miscible states are analytically developed by means of the Flory–Huggins solution theory and solubility parameter. The quantitative bottom and upper solubility limits for a total of 13 binary and ternary mixtures are calculated at different conditions. Moreover, the composition, temperature and pore radius are specifically studied to evaluate their effects on the soluble and miscible states. On the basis of the work from this study, the insoluble, soluble but immiscible, and miscible states are definitively quantified and clearly distinguished for the first time.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.938
Threshold uncertainty score0.268

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.224
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2020
Admission routes1
Has abstractyes

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