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Record W3014274645 · doi:10.1039/d0cp01518k

Quantitative structure–property relationship of the photoelectrochemical oxidation of phenolic pollutants at modified nanoporous titanium oxide using supervised machine learning

2020· article· en· W3014274645 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenuePhysical Chemistry Chemical Physics · 2020
Typearticle
Languageen
FieldEnvironmental Science
TopicWater Quality Monitoring and Analysis
Canadian institutionsUniversity of Guelph
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsNanoporousOxideTitanium oxideTitaniumPollutantMaterials scienceProperty (philosophy)Chemical engineeringChemistryNanotechnologyMetallurgyOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

Here we report on an advanced photoelectrochemical (PEC) oxidation of 22 phenolic pollutants based on modified nanoporous TiO2, which was directly grown on a titanium substrate electrochemically. Their degradation rate constants were experimentally determined and their physicochemical properties were computaionally calculated. The quantitative structure-property relationship (QSPR) was elucidated by employing multiple linear regression (MLR) method. A supervised machine learning approach was employed to build QSPR models. The high predictive abilities of the QSPR model were validated via leave-one-out (LOO) method and a strict regimen of statistical validation tests. The significant descriptors identified in the QSPR Model for the phenolic compounds were also assessed using a typical dye pollutant Rhodamine B, further confirming the high effectiveness and predictability of the optimized model. Our study has shown that the integrated effect of the structural, hydrophobic and topological properties along with electronic property should be considered in order to design an efficient PEC catalytic approach for environmental applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.060
Threshold uncertainty score0.640

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.041
GPT teacher head0.251
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it