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Record W3018919816 · doi:10.1002/mren.202000004

Straightforward Synthesis and Evaluation of Polymeric Sensing Materials for Acetone Detection

2020· article· en· W3018919816 on OpenAlexafffund
Alison J. Scott, Noushin Majdabadifarahani, Katherine M. E. Stewart, Thomas A. Duever, Alexander Penlidis

Bibliographic record

VenueMacromolecular Reaction Engineering · 2020
Typearticle
Languageen
FieldEngineering
TopicAdvanced Chemical Sensor Technologies
Canadian institutionsToronto Metropolitan UniversityUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsSorptionPolypyrroleAcetonePolyanilineChemistryAnalyteSolventPolymerPolymer chemistryChemical engineeringInorganic chemistryOrganic chemistryChromatographyAdsorptionPolymerization

Abstract

fetched live from OpenAlex

Abstract Three polymeric materials (polyaniline, polypyrrole, and poly(methyl methacrylate)) are selected, prepared, and evaluated for potential use in acetone sensing (for possible diabetes‐related applications). Of the materials studied, polyaniline and polypyrrole show the most promise. Polypyrrole allows for more acetone sorption (i.e., higher concentration of acetone sorbed), but does not distinguish between different target analytes (that is, it is not selective). A material's ability to distinguish between several gas analytes simultaneously (in a gas mixture) is rarely evaluated; selectivity is typically based on a “one‐analyte‐at‐a‐time” investigation. However, comparison of acetone sorption (in one experimental test) and interferent sorption (in a complementary experimental test) does not consider interactions that might occur between gas analytes; this motivates the sorption analysis of gas mixtures that is shown in this work. The most promising results are obtained when polyaniline or polypyrrole is exposed to acetone‐rich gas mixtures with low amounts of acetaldehyde, ethanol, and benzene (interferent gases). Polymer doping using three metal oxides (SnO 2 , WO 3 , and ZnO) is also investigated, but metal oxide addition has a limited effect on the sorption performance. This is true for all three metal oxides, regardless of the amount of doping (over the range studied; up to 20 wt%).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.196
Threshold uncertainty score0.636

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.222
Teacher spread0.207 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2020
Admission routes2
Has abstractyes

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