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Record W3025264384 · doi:10.11575/prism/37848

Process Simulation of Methanol Production from Water Electrolysis and Tri-Reforming

2020· dissertation· en· W3025264384 on OpenAlexfundno aff
Chenxu Shi

Bibliographic record

VenuePRISM (University of Calgary) · 2020
Typedissertation
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsElectrolysisProcess engineeringEnvironmental scienceProcess (computing)Production (economics)MethanolHydrogen productionProcess simulationElectrolysis of waterWaste managementEngineeringComputer scienceChemistryEconomicsCatalysisOperating systemMicroeconomics

Abstract

fetched live from OpenAlex

The alarmingly increase in anthropogenic CO2 emissions is widely considered as the root cause of global warming. To mitigate this issue, CO2 utilization via methanol production can be an effective approach. The present study develops an innovative process to produce methanol by combining water electrolysis with tri-reforming of methane (TRM). The proposed process utilizes carbon-free electricity to split water into O2 and H2; O2 is collected for partial oxidation reaction in the TRM and H2 is collected for stoichiometric number (SN) optimization. This process configuration eliminates the typical problem of H2 deficiencies associated with methanol synthesis and allows for additional CO2 to be converted. The main process flowsheet is developed with the well-known Aspen HYSYS process simulator. Then the feasibility of this project is evaluated based on its techno-economic performance as well as greenhouse gas (GHG) emissions. The estimated capital expenditure (CAPEX), operating expenditure (OPEX) and GHG emissions of the baseline plant are $774 million, $263 million/year and -0.14 kgCO2eq/kgMeOH, respectively. In particular, water electrolysis process accounts for 34% of CAPEX and 54% of OPEX. A discounted cash flow (DCF) model combined with sensitivity analyses show that a breakeven point can be reached with a methanol price of $491/ton. The results from this study demonstrate that combining water electrolysis with TRM can improve the sustainability and economic viability for methanol production. However, in order for the process to become more financially attractive, further research and development are necessary to drive down the costs of the current water electrolysis technology.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.100
Threshold uncertainty score0.872

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.212
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

Explore more

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