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Co-processing of Hydrothermal Liquefaction Biocrude with Vacuum Gas Oil through Hydrotreating and Hydrocracking to Produce Low-Carbon Fuels

2020· article· en· W3030022754 on OpenAlexafffund
Sandeep Badoga, Anton Alvarez‐Majmutov, Tingyong Xing, Rafał Gieleciak, Jinwen Chen

Bibliographic record

VenueEnergy & Fuels · 2020
Typearticle
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsNatural Resources Canada
FundersGovernment of Canada
KeywordsHydrodesulfurizationHydrothermal liquefactionNaphthaDiesel fuelJet fuelVacuum distillationUltra-low-sulfur dieselChemistryCo-processingFluid catalytic crackingCarbon fibersChemical engineeringFuel oilCrackingPulp and paper industryWaste managementSulfurOrganic chemistryMaterials scienceCatalysisDistillation

Abstract

fetched live from OpenAlex

In this study, we investigate the potential of co-processing hydrothermal liquefaction (HTL) biocrude with vacuum gas oil (VGO) in a hydrocracking process with hydrotreating as the first step. Experiments were conducted in a continuous hydroprocessing pilot plant in two stages: hydrotreating and hydrocracking. Two feeds were tested: first pure VGO to establish a baseline and then a co-processing blend having 7.5 vol % HTL biocrude. In the first stage, the VGO and co-processing blend were sequentially hydrotreated to meet the quality specification of the hydrocracking catalyst. The second stage consisted of hydrocracking the two hydrotreated products from the first stage, and the resulting products were distilled into naphtha, diesel, and jet fuel fractions for characterization. The hydrotreating step achieved satisfactory sulfur and nitrogen removal levels for both feeds, but it was ineffective in converting oxygen compounds in the co-processing blend, resulting in a product with 1530 ppmw oxygen. During hydrocracking, the co-processing blend required a higher reaction temperature than the baseline VGO to achieve the same conversion level, a behavior attributed to the oxygen and nitrogen levels in the co-processing blend after hydrotreating. Despite these effects, overall product distribution and hydrogen consumption for both scenarios were quite comparable. Characterization of hydrocracked products showed only subtle differences in quality and hydrocarbon type composition, while biogenic carbon measurements revealed that the majority of biogenic carbon is transferred to the naphtha, diesel, and jet fuel fractions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.023
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.211
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations52
Published2020
Admission routes2
Has abstractyes

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