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Record W3034112315 · doi:10.1002/admi.201901870

Structure‐Dependent Wear and Shear Mechanics of Nanostructured MoS<sub>2</sub> Coatings

2020· article· en· W3034112315 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Materials Interfaces · 2020
Typearticle
Languageen
FieldEngineering
TopicMetal and Thin Film Mechanics
Canadian institutionsCanada Research ChairsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaMitacsUniversity of Toronto
KeywordsMaterials sciencevan der Waals forceComposite materialLubricantNanostructureFracture mechanicsNanoindentationNanocrystalline materialTribologyShear (geology)Fracture toughnessNanotechnology

Abstract

fetched live from OpenAlex

Abstract Sputter‐deposited molybdenum disulfide coatings are one of the most common lubricants for extreme environments. However, their performance predictability remains limited by the complexity of van der Waals wear and shear mechanics in bulk materials resulting in unexpected premature failure. In the present study, two nanostructured MoS 2 coatings of similar macroscopic properties are shown to exhibit entirely different wear and shear mechanics due to their nanostructure. Friction force microscopy with steel‐beaded cantilevers is used to measure the per‐cycle evolution of friction, wear, and topography in situ over the lubricant lifetime under an inert nitrogen environment. Molecular dynamics simulations confirm the subsurface structural failure mechanisms of the coatings under shear stress, and atomic force microscope phase imaging and Raman spectroscopy are used to identify tribofilm formation mechanics. The nanocrystal–amorphous composite structure shows improved wear resistance but at the cost of limited stress relaxation which creates high‐stress failure and fracture‐dominated wear. The purely nanocrystalline coating exhibits lower shear resistance but consistent stress relaxation by van der Waals cleavage and triple junction fracture which results in higher wear rates with predictable abrasion‐dominated failure. The contrast in nanoscale performance of the coatings allows for the lubricant nanostructure to be tuned for ideal applications for extreme environments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.939

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.191
Teacher spread0.184 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it