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Record W3036245508 · doi:10.1002/chem.202000072

Building Hierarchical Microcubes Composed of One‐Dimensional CoSe<sub>2</sub>@Nitrogen‐Doped Carbon for Superior Sodium Ion Batteries

2020· article· en· W3036245508 on OpenAlexaff
Tiezhong Liu, Youpeng Li, Shuang Hou, Chenghao Yang, Yayun Guo, Tian Sheng, Lingzhi Zhao

Bibliographic record

VenueChemistry - A European Journal · 2020
Typearticle
Languageen
FieldEngineering
TopicAdvancements in Battery Materials
Canadian institutionsInstitute of Aging
FundersScience and Technology Planning Project of Guangdong ProvinceNational Natural Science Foundation of China
KeywordsCarbon fibersDopingMaterials scienceSodiumNitrogenIonNanotechnologyEngineering physicsOptoelectronicsComposite materialChemistryEngineeringComposite numberMetallurgy

Abstract

fetched live from OpenAlex

Abstract Designing and synthesizing highly stable anode materials with high capacity is critical for the practical application of sodium ion batteries (SIBs), however, to date, this remains an insurmountable barrier. The introduction of hierarchical architectures and carbon supports is proving an effective strategy for addressing these challenges. Thus, we have fabricated a hierarchical CoSe2@nitrogen‐doped carbon (CoSe2@NC) microcube composite using the Prussian blue analogue Co3[Co(CN)6]2 as template. The rational combination of the unique hierarchical construction from one to three dimensions and a nitrogen‐doped carbon skeleton facilitates sodium ion and electron transport as well as stabilizing the host structure during repeated discharge/charge processes, which contributes to its excellent sodium storage capability. As expected, the as‐prepared CoSe2@NC composite delivered remarkable reversible capacity and ultralong cycling lifespan even at a high rate of 2.0 A g−1 (384.3 mA h g−1 after1800 loops) when serving as the anode material for SIBs. This work shows the great potential of the CoSe2‐based anode for practical application in SIBs, and the original strategy may be extended to other anode materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.218
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2020
Admission routes1
Has abstractyes

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Same venueChemistry - A European JournalSame topicAdvancements in Battery MaterialsFrench-language works237,207