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Record W3036811792 · doi:10.1038/s41467-020-20408-5

Giant topological longitudinal circular photo-galvanic effect in the chiral multifold semimetal CoSi

2021· article· en· W3036811792 on OpenAlexaff
Zhuoliang Ni, K. Wang, Yang Zhang, Óscar Pozo, Bîng Xu, Xingyue Han, Kaustuv Manna, Johnpierre Paglione, Claudia Felser, Adolfo G. Grushin, Fernando de Juan, E. J. Melé, Liang Wu

Bibliographic record

VenueNature Communications · 2021
Typearticle
Languageen
FieldPhysics and Astronomy
TopicTopological Materials and Phenomena
Canadian institutionsCanadian Institute for Advanced Research
FundersArmy Research OfficeBasic Energy SciencesDivision of Materials ResearchAgencia Estatal de InvestigaciónMultidisciplinary University Research InitiativeMaterials Research Science and Engineering Center, Harvard UniversityMax-Planck-GesellschaftDeutsche ForschungsgemeinschaftU.S. Department of DefenseU.S. Department of EnergyEuropean CommissionAgence Nationale de la RechercheGordon and Betty Moore FoundationMinisterio de Ciencia, Innovación y UniversidadesMinisterio de Educación, Cultura y DeporteUniversity of PennsylvaniaSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen ForschungNational Science Foundation
KeywordsPhotocurrentCircular polarizationSemimetalPhysicsTopology (electrical circuits)Condensed matter physicsQuantization (signal processing)PhotonChirality (physics)Polarization (electrochemistry)Band gapMaterials scienceOptoelectronicsChiral anomalyOpticsQuantum mechanicsChemistryFermion

Abstract

fetched live from OpenAlex

Abstract The absence of mirror symmetry, or chirality, is behind striking natural phenomena found in systems as diverse as DNA and crystalline solids. A remarkable example occurs when chiral semimetals with topologically protected band degeneracies are illuminated with circularly polarized light. Under the right conditions, the part of the generated photocurrent that switches sign upon reversal of the light’s polarization, known as the circular photo-galvanic effect, is predicted to depend only on fundamental constants. The conditions to observe quantization are non-universal, and depend on material parameters and the incident frequency. In this work, we perform terahertz emission spectroscopy with tunable photon energy from 0.2 –1.1 eV in the chiral topological semimetal CoSi. We identify a large longitudinal photocurrent peaked at 0.4 eV reaching ~550 μ A/V 2 , which is much larger than the photocurrent in any chiral crystal reported in the literature. Using first-principles calculations we establish that the peak originates only from topological band crossings, reaching 3.3 ± 0.3 in units of the quantization constant. Our calculations indicate that the quantized circular photo-galvanic effect is within reach in CoSi upon doping and increase of the hot-carrier lifetime. The large photo-conductivity suggests that topological semimetals could potentially be used as novel mid-infrared detectors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.300
Teacher spread0.279 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations168
Published2021
Admission routes1
Has abstractyes

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