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Record W3037180799 · doi:10.3390/suschem1010006

Process Intensification of Dichlorodiphenyltrichloroethane Detection Methods for Determining Trace Concentrations in Soils

2020· article· en· W3037180799 on OpenAlex
Jinghan Zhao, Stephen Vanderburgt, Rafael M. Santos, Yi Wai Chiang

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
aboutThe title or abstract carries a Canadian signal from the geographic lexicon.

Bibliographic record

VenueSustainable Chemistry · 2020
Typearticle
Languageen
FieldEnvironmental Science
TopicToxic Organic Pollutants Impact
Canadian institutionsUniversity of Guelph
FundersOntario Ministry of Agriculture, Food and Rural Affairs
KeywordsExtraction (chemistry)Soil waterEnvironmental scienceResidue (chemistry)Ultrasonic sensorChemistryYield (engineering)Soil testPesticideEnvironmental chemistryPulp and paper industrySoil scienceChromatographyMaterials scienceAgronomyMetallurgyEngineering

Abstract

fetched live from OpenAlex

Dichlorodiphenyltrichloroethane (DDT) residue in Ontario soil is expected to be found at trace levels, since it has been banned for over 45 years in Canada. This presents challenges to the efficiency and accuracy of conventional detection methods. This study intensified the conventional DDT detection method, in the characterization of aged soil samples collected from historically-treated sites in Ontario. Recovery, time consumption, and labor intensity were considered for the intensification evaluation. Ultrasonic probe extraction was found to significantly shorten the extraction time, with similar yield compared to ultrasonic water bath extraction and homogenized extraction. Homogenized extraction for 24 h following ultrasonic probe extraction can increase yield over 27%. Rotary evaporator concentration was used, since it can reduce the operating time with comparable recovery. The Florisil clean-up column used in the conventional method was removed from the intensified method, due to its negligible effect and high time consumption. The intensified method may be valuable for further investigation to determine other trace level organochlorine pesticide residues in soil samples.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.068
Threshold uncertainty score0.543

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.308
Teacher spread0.292 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it