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Record W3039356924 · doi:10.1103/physreve.101.062706

Rodlike molecules in extreme confinement

2020· article· en· W3039356924 on OpenAlexafffund
Xiaomei Yao, Jeff Z. Y. Chen

Bibliographic record

VenuePhysical review. E · 2020
Typearticle
Languageen
FieldMaterials Science
TopicPickering emulsions and particle stabilization
Canadian institutionsUniversity of Waterloo
FundersPostdoctoral Science Foundation of Jiangsu ProvinceNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of China
KeywordsRigidity (electromagnetism)Length scaleMoleculeChemical physicsCondensed matter physicsLiquid crystalMaterials scienceCrystal (programming language)Molecular dynamicsPhysicsQuantum mechanics

Abstract

fetched live from OpenAlex

A unique feature of colloid particles and biopolymers is the molecule's intrinsic rigidity characterized by a molecular-level length scale. Under extreme confinement conditions at cellular scales or in nanodevices, these molecules can display orientational ordering accompanied by severe density depletion. Conventional liquid-crystal theories, such as the Oseen-Frank or Landau-de Gennes theories, cannot capture the essential molecular-level properties: the boundary effects, which extend to a distance of the rigidity length scale, and the drastic variations of the inhomogeneous molecular density. Here we show, based on a simple interpretation of the Onsager model, that rodlike molecules in extreme annular confinement produce unusual liquid-crystal defect structures that are independent phases from the patterns usually seen in a weaker confinement environment.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.337
Threshold uncertainty score0.549

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.091
GPT teacher head0.327
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2020
Admission routes2
Has abstractyes

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