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Record W3039405582 · doi:10.1021/acsanm.0c01286

PdO Nanoparticles Supported on MnO<sub>2</sub> Nanowire Aerogels as Catalysts for Low-Temperature Methane Combustion

2020· article· en· W3039405582 on OpenAlexafffund
Yiling Dai, Haiyan Wang, Shida Liu, Mark J. MacLachlan, Michael O. Wolf, Kevin J. Smith

Bibliographic record

VenueACS Applied Nano Materials · 2020
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsUniversity of British Columbia
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of British ColumbiaCanada Foundation for Innovation
KeywordsMethaneCatalysisAerogelNanoparticleChemical engineeringMaterials scienceNanomaterialsHydrothermal circulationCatalytic combustionSpace velocityCombustionInorganic chemistryNanotechnologyChemistrySelectivityOrganic chemistry

Abstract

fetched live from OpenAlex

Palladium oxide nanoparticles were loaded onto a nanostructured MnO2 aerogel by a deposition–precipitation method. The resulting nanomaterial exhibited excellent catalytic activity for low-temperature methane combustion, achieving complete methane conversion to CO2 at 330 °C (GHSV = 180000 mL/(g h)). The enhanced activity is attributed to excellent reducibility and exposure of active PdO facets. The hydrothermal stability of the composite catalyst was improved, and the deactivation mechanism was explored. These novel catalysts form free-standing monoliths and could be useful in natural gas vehicles and other methane scrubbing applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.244
Teacher spread0.230 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2020
Admission routes2
Has abstractyes

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