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Record W3042597418 · doi:10.1021/acs.est.0c04114

Broad Exposure of the North American Environment to Phenolic and Amino Antioxidants and to Ultraviolet Filters

2020· article· en· W3042597418 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

aboutThe title or abstract carries a Canadian signal from the geographic lexicon.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueEnvironmental Science & Technology · 2020
Typearticle
Languageen
FieldEnvironmental Science
TopicIndoor Air Quality and Microbial Exposure
Canadian institutionsnot available
FundersU.S. Environmental Protection Agency
KeywordsDiphenylamineEnvironmental chemistryEnvironmental scienceSedimentChemistryOrganic chemistryBiology

Abstract

fetched live from OpenAlex

The present study provides a comprehensive investigation of three suites of commonly used synthetic additives: phenolic and amino antioxidants and ultraviolet filters. The concentrations of 47 such compounds and their transformation products were measured in 20 atmospheric particle samples collected in Chicago, in 21 Canadian e-waste dust samples, in 32 Canadian and United States’ residential dust samples, and in 10 sediment samples collected from the Chicago Sanitary and Ship Canal. Despite their large production volumes in the United States, environmental data on antioxidants and UV filters in North America is limited. These compounds were detected in all the samples, indicating their ubiquitous distribution in the North American environment. The most prevalent compounds were 2,6-di-t-butyl-p-benzoquinone, diphenylamine, 4,4′-di-t-octyl diphenylamine, 2,4-dihydroxybenzophenone, and 2-hydroxy-4-methoxybenzophenone. The e-waste dust contained significantly greater total concentrations of these compounds than the Canadian residential dust, while intermediate levels were detected in the United States residential dust. The sediment samples showed relatively high levels of N,N′-diphenylbenzidine, the source of which is unclear, and some benzotriazole UV filters. Daily intake rates by dust ingestion for these compounds ranged from 1–10 ng/(kg·day) for adults to 10–100 ng/(kg·day) for toddlers. Due to the wide distribution of these compounds in both the ambient and built environments, future research on their potential toxic effects on people and ecosystems is important.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesScience and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.523
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.004
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.195
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it