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Record W3043542522 · doi:10.1149/1945-7111/aba6c8

A New Method for Corrosion Current Measurement: the Dual-Electrochemical Cell (DEC)

2020· article· en· W3043542522 on OpenAlexaff
Dan Guo, Mingyu Li, Jiju M. Joseph, J.C. Wren

Bibliographic record

VenueJournal of The Electrochemical Society · 2020
Typearticle
Languageen
FieldMaterials Science
TopicCorrosion Behavior and Inhibition
Canadian institutionsWestern University
Fundersnot available
KeywordsAlgorithmComputer science

Abstract

fetched live from OpenAlex

This paper presents the “dual electrochemical cell” (DEC) method, a new technique that allows monitoring of corrosion current ( <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>i</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> </mml:math> ) in real time with a corrosion potential <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mfenced close=")" open="(" separators=""> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>E</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> </mml:mrow> </mml:mfenced> </mml:math> that may change with time. In this method, the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>E</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> </mml:math> of a metal corroding in a solution containing the oxidant of interest is measured in the 1 st cell. This potential is then continuously applied in real time to a second cell using the same metal electrode in the same solution but free of the oxidant, and the current of the 2 nd cell, which represents the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>i</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> </mml:math> of the 1 st cell, is monitored. This setup allows direct measurement of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>i</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> </mml:math> without having to polarize the corroding electrode away from <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>E</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> <mml:mo>.</mml:mo> </mml:math> The advantages of DEC over conventional methods are that it does not require the corroding system to be at steady state, and avoids any ambiguities associated with the extrapolation of the measured current-potential relationship to extract <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>i</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> <mml:mo>.</mml:mo> </mml:math> The <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>i</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> </mml:math> values obtained using the DEC method were compared with those obtained using conventional polarization techniques, using dissolved metal concentrations and surface analysis observations, and the results showed that the DEC method provides the most accurate measurement of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msub> <mml:mrow> <mml:mi>i</mml:mi> </mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">corr</mml:mi> </mml:mrow> </mml:msub> <mml:mo>.</mml:mo> </mml:math>

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: none
Teacher disagreement score0.900
Threshold uncertainty score0.434

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.033
GPT teacher head0.293
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2020
Admission routes1
Has abstractyes

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