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Lithium diffusion in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>Li</mml:mi><mml:mi>Mn</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:msub><mml:mrow><mml:mi mathvariant="normal">O</mml:mi></mml:mrow><mml:mn>4</mml:mn></mml:msub></mml:math> detected with <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msup><mml:mi>μ</mml:mi><mml:mo>±</mml:mo></mml:msup><mml:mi>SR</mml:mi></mml:math>

2020· article· lv· W3046126991 on OpenAlexaff
Jun Sugiyama, Ola Kenji Forslund, Elisabetta Nocerino, Nami Matsubara, Konstantinos Papadopoulos, Yasmine Sassa, Stephen P. Cottrell, A. D. Hillier, Katsuhiko Ishida, Martin Må̊nsson, J. H. Brewer

Bibliographic record

VenuePhysical Review Research · 2020
Typearticle
Languagelv
FieldEngineering
TopicAdvancements in Battery Materials
Canadian institutionsUniversity of British ColumbiaTRIUMF
FundersJapan Society for the Promotion of ScienceVetenskapsrådetStiftelsen för Strategisk Forskning
KeywordsDiffusionPhysicsThermodynamics

Abstract

fetched live from OpenAlex

Positive-and negative-muon spin rotation and relaxation ( SR) was first used to investigate fluctuations of nuclear magnetic fields in an olivine-type battery material, LiMnPO 4 , in order to clarify the diffusive species, namely, to distinguish between a + hopping among interstitial sites and Li + ions diffusing in the LiMnPO 4 lattice. Muon diffusion can only occur in + SR, because the implanted -forms a stable muonic atom at the lattice site, and therefore any change in linewidth measured with -SR must be due to Li + diffusion. Since the two measurements exhibit a similar increase in the field fluctuation rate with temperature above 100 K, it is confirmed that Li + ions are in fact diffusing. The diffusion coefficient of Li + at 300 K and its activation energy were estimated to be 1.4(3) 10 -10 cm 2 /s and 0.19(3) eV, respectively. Such combined SR measurements are thus shown to be a suitable tool for detecting ion diffusion in solid-state energy materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.008
metaresearch head score (Gemma)0.007
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Open science, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Science and technology studies, Open science, Research integrity, Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.861
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0080.007
Meta-epidemiology (narrow)0.0040.006
Meta-epidemiology (broad)0.0020.005
Bibliometrics0.0020.006
Science and technology studies0.0050.005
Scholarly communication0.0050.005
Open science0.0090.010
Research integrity0.0060.008
Insufficient payload (model declined to judge)0.2700.014

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.273
Teacher spread0.246 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2020
Admission routes1
Has abstractyes

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