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Record W3046182198 · doi:10.14447/jnmes.v22i4.a01

An Improved Hydroxide Conversion Process of Anionic Exchange Membranes for Alka-line Fuel Cells

2019· article· en· W3046182198 on OpenAlexafffundvenue
Lin Xie, Donald W. Kirk

Bibliographic record

VenueJournal of New Materials for Electrochemical Systems · 2019
Typearticle
Languageen
FieldEngineering
TopicFuel Cells and Related Materials
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaQueen's University
KeywordsHydroxideMembraneProcess (computing)ChemistryLine (geometry)Chemical engineeringFuel cellsInorganic chemistryComputer scienceBiochemistryEngineeringOperating systemMathematics

Abstract

fetched live from OpenAlex

Robust anionic exchange membranes (AEMs) are needed for alkaline fuel cells (AFCs) [1].To convert the as-produced AEMs to hydroxide form, conventionally an one step high alkalinity 1-2M alkaline solution for 24 -48hrs is used [1].However, this high alkalinity process will be shown to limit the ion exchange capacity and reduce long term viability of the AEMs.To investigate the degradation process, short-term activation and longterm stability of 3 AEMs were studied.Short-term degradation was found to be caused by the high concentration of hydroxide ions in the initial conversion process.Long-term degradation was found to be caused by the substituted hydroxide ions which caused gradual loss of conducting species from the membrane.A modification of the conventional one step high alkalinity process was developed to mitigate this membrane degradation.This modified process used multi-step low alkalinity conversion stages.Three types of commercial AEM products from Fumatech (FAS-PP-75, FAA-3-PK-130, and FAD-55) were compared with both the conventional and modified processes.The results showed that the multistep low alkalinity process improved the initial membrane performances by at least 20%.The long-term stability was substantially enhanced for FAS-PP-75 and FAA-3-PK-130.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.223
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations1
Published2019
Admission routes3
Has abstractyes

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Same venueJournal of New Materials for Electrochemical SystemsSame topicFuel Cells and Related MaterialsFrench-language works237,207