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Record W3081206324 · doi:10.1021/acs.jpcc.0c06338

Effect of Sodium Citrate and Calcium Ions on the Spontaneous Displacement of Heavy Oil from Quartz Surfaces

2020· article· en· W3081206324 on OpenAlexafffund
Bailin Xiang, Rui Li, Bo Liu, Rogério Manica, Qingxia Liu

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2020
Typearticle
Languageen
FieldEngineering
TopicEnhanced Oil Recovery Techniques
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaSyncrude
KeywordsQuartzAsphaltDisplacement (psychology)IonDissolutionDewettingSurface tensionChemistryMaterials scienceContact angleMineralogyChemical engineeringWettingComposite materialOrganic chemistryThermodynamics

Abstract

fetched live from OpenAlex

Abstract The dynamic displacement of heavy oil from solid surfaces by water plays a significant role in the oil recovery process. In this work, a bitumen–water–quartz system was applied to study the effect of sodium citrate (Na3Cit) and calcium ions (Ca2+) on the dynamic displacement of bitumen from quartz surfaces. It was found that the addition of Ca2+ slowed down the bitumen displacement rate and generated daughter droplets during the receding process. In contrast, the presence of Na3Cit not only accelerated the displacement of bitumen from quartz surfaces but also led to a smaller water contact angle at the end of the experiments. Moreover, Ca2+ ions were chelated by the added Na3Cit, which counterbalanced the detrimental effect of Ca2+ on the bitumen displacement. The reduced interfacial tension of the bitumen–water interface and the increased negative charges on both bitumen and silica surfaces by Na3Cit were considered as the reasons for the improved bitumen displacement process. To better understand the underlying physics, both the hydrodynamic (HD) model and the molecular kinetic (MK) model were employed to analyze the dewetting dynamics of heavy oil from quartz surfaces under the effect of Ca2+ and Na3Cit.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.229
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2020
Admission routes2
Has abstractyes

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