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Record W3082200404 · doi:10.1002/cem.3299

Partial least squares discrimination applied to a few samples dataset: A case for predicting the presence of pesticide in lettuce

2020· article· en· W3082200404 on OpenAlex
Sílvio José de Souza, Patrícia Valderrama, Nelson Consolin Filho, Eduardo Jorge Pilau, Ailey Aparecida Coelho Tanamati, Peter D. Wentzell, Paulo Henrique Março

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Chemometrics · 2020
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicPesticide Residue Analysis and Safety
Canadian institutionsDalhousie University
FundersConselho Nacional de Desenvolvimento Científico e TecnológicoCoordenação de Aperfeiçoamento de Pessoal de Nível Superior
KeywordsPartial least squares regressionLinear discriminant analysisStatisticsReliability (semiconductor)MathematicsComputer scienceWilcoxon signed-rank testPattern recognition (psychology)Artificial intelligence

Abstract

fetched live from OpenAlex

Abstract To perform discriminant analysis through partial least squares (PLS‐DA), it is important to note that the smaller the set of samples and the higher the variable to sample ratio, the higher the chance of a too optimistic classification model. In this sense, it is necessary to use strategies to check for the possibility that the classification achieved is done by chance. In metabolomics studies, it is not uncommon to work with a reduced number of samples, in which discrimination approaches must be evaluated according to its reliability. Considering this issue, this study aimed to show a case study to deal with few samples using PLS‐DA to discriminate lettuce cultivated in the absence and presence of imidacloprid (IMI). The data were acquired by using ultra‐high‐performance liquid chromatography coupled to a quadrupole‐time of flight mass spectrometry, and the model prediction ability was evaluated by permuting the classes. The performance of the PLS‐DA model built using all the variables reached 100% correct classification. Nonetheless, the reliability tests (Wilcoxon, sign test, and Rand t test) indicated that the model has been build choosing variables by chance. By using the variable importance in projection, it was possible to build a model with reliable specificity and sensitivity equals 1. The study showed the need to check the classification ability in PLS‐DA models through strategies such as variable selection and the permutation test in order to allow for the evaluation of the reliability of the results, even in cases in which the classification reaches 100% in the target.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.004
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.696
Threshold uncertainty score0.429

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.004
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.072
GPT teacher head0.285
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it