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Experimental Evaluation and Empirical Modeling of Cross-Flow Microfiltration for Solids and Ash Removal from Fast Pyrolysis Bio-Oil

2020· article· en· W3082294401 on OpenAlexafffund
Dillon Mazerolle, Benjamin Bronson, Boguslaw Kruczek

Bibliographic record

VenueEnergy & Fuels · 2020
Typearticle
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsUniversity of OttawaNatural Resources Canada
FundersOffice of Energy Research and Development
KeywordsMicrofiltrationPyrolysisFiltration (mathematics)CharMaterials scienceWaste managementChemical engineeringPulp and paper industryProcess engineeringEnvironmental scienceChemistryMembrane

Abstract

fetched live from OpenAlex

Abstract The presence of suspended char particulate and ash in fast pyrolysis bio-oil produced from the fast pyrolysis of high ash forestry materials poses a significant technical challenge for the direct utilization and/or catalytic upgrading of these low-carbon renewable fuels. Cross-flow microfiltration is a physical upgrading process strategy that can remove suspended solids and ash from the fast pyrolysis bio-oil. To develop data sets on operational characteristics of fast pyrolysis bio-oil cross-flow microfiltration, experimental research was undertaken. Using a variety of filtration media with nominal pore sizes between 1 and 40 μm, typical solids and ash rejection ranged from 80 to 95% and 4–45%, respectively. An empirical modeling procedure was developed to predict the throughput and resistance associated with cross-flow microfiltration of fast pyrolysis bio-oil, which demonstrated good agreement with generated experimental data. Key operating parameters were also studied, and it was found that transmembrane pressures less than 1 bar and fluid preheat temperatures up to 60 °C were ideal for maximizing the pseudo steady-state flux of the process. Furthermore, the use of low viscosity, miscible solvents, and/or initial solids reduction pathways prior to microfiltration offered additional routes to potentially improve the throughput of such a process.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.016

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.030
GPT teacher head0.280
Teacher spread0.251 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2020
Admission routes2
Has abstractyes

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