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Impedimetric Detection of Bacteria Using Hierarchical 3D Nanostructured Gold

2020· article· en· W3082355270 on OpenAlexaff
Alireza Sanati, Roozbeh Siavash Moakhar, Mahsa Jalali, Tamer AbdElFatah, Sarah Elizabeth Flynn, Sahar Sadat Mahshid, Sara Mahshid

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldEngineering
TopicBiosensors and Analytical Detection
Canadian institutionsSunnybrook Health Science CentreHealth Sciences CentreMcGill University
Fundersnot available
KeywordsDielectric spectroscopyDetection limitBacteriaColloidal goldAnalyteNanotechnologyMaterials scienceNanostructureSpectroscopyElectrical impedanceElectrochemistryAnalytical Chemistry (journal)ChemistryNanoparticleChromatographyBiologyPhysicsElectrode

Abstract

fetched live from OpenAlex

Impedimetric electrochemical sensing offers direct, label-free, cost-effective, accurate, and rapid detection of biological analytes. Among different types of nanostructured platforms, hierarchical structures of gold have proven to be beneficial for impedimetric and direct diagnosis of bacteria. In this research, a two-step electrodeposition method was used to achieve hierarchical nanostructures of gold for impedimetric distinction of E. coli-k12. The current observations demonstrate that the two-step electrodeposition method can convert sharp and needle-shaped structures of gold into curved and smooth structures that are able to detect bacteria, with enhanced sensitivity. The results of Electrochemical impedance spectroscopy (EIS) showed a limit of detection of approximately 90 CFU in 30 μl of solution and a linear range of detection between 3×103and 3×107CFU mL-1 for the final sensor. In addition, this structure can detect bacteria in less than 10 minutes. Ultimately, this ultrasensitive label-free bacteria sensor, based on a novel engineered hybrid method, opens interesting avenues in bacteria sensing with exciting detection abilities. Keywords: E. coli bacteria, electrodeposition, hierarchical nanostructures of gold, electrochemical impedance spectroscopy (EIS).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.201
Teacher spread0.188 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2020
Admission routes1
Has abstractyes

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