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Record W3083193338 · doi:10.1002/adfm.202004612

Epitaxial Metal Halide Perovskites by Inkjet‐Printing on Various Substrates

2020· article· en· W3083193338 on OpenAlexaff
Mykhailo Sytnyk, AmirAbbas YousefiAmin, Tim Freund, Annemarie Prihoda, Klaus Götz, Tobias Unruh, Christina Harreiß, Johannes Will, Erdmann Spiecker, Andres Osvet, Christoph J. Brabec, Ulrike Künecke, Peter J. Wellmann, Valentine V. Volobuev, Jędrzej Korczak, A. Szczerbakow, T. Story, Clemens Simbrunner, G. Springholz, Daniel Wechsler, Ole Lytken, Sebastian Lotter, Felix Kampmann, Janina Maultzsch, Kamalpreet Singh, Oleksandr Voznyy, Wolfgang Heiß

Bibliographic record

VenueAdvanced Functional Materials · 2020
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsThe Scarborough HospitalUniversity of Toronto
FundersTechnische Universität BerlinAustrian Science FundFundacja na rzecz Nauki PolskiejDeutsche Forschungsgemeinschaft
KeywordsMaterials scienceEpitaxyHalideThin filmNanotechnologyPerovskite (structure)SemiconductorNanostructureOptoelectronicsCadmium telluride photovoltaicsChemical engineeringInorganic chemistryLayer (electronics)

Abstract

fetched live from OpenAlex

Abstract Metal‐halide‐perovskites revolutionized the field of thin‐film semiconductor technology, due to their favorable optoelectronic properties and facile solution processing. Further improvements of perovskite thin‐film devices require structural coherence on the atomic scale. Such perfection is achieved by epitaxial growth, a method that is based on the use of high‐end deposition chambers. Here epitaxial growth is enabled via a ≈1000 times cheaper device, a single nozzle inkjet printer. By printing, single‐crystal micro‐ and nanostructure arrays and crystalline coherent thin films are obtained on selected substrates. The hetero‐epitaxial structures of methylammonium PbBr3 grown on lattice matching substrates exhibit similar luminescence as bulk single crystals, but the crystals phase transitions are shifted to lower temperatures, indicating a structural stabilization due to interfacial lattice anchoring by the substrates. Thus, the inkjet‐printing of metal‐halide perovskites provides improved material characteristics in a highly economical way, as a future cheap competitor to the high‐end semiconductor growth technologies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.201
Teacher spread0.187 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations30
Published2020
Admission routes1
Has abstractyes

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