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TROPOMI SO2 column retrievals: validation, inter-comparison with other satellite data sets and algorithm evolution

2020· article· en· W3083276758 on OpenAlexaff
Nicolas Theys, Can Li, N. A. Krotkov, Isabelle De Smedt, Christophe Lerot, Huan Yu, Jonas Vlietinck, Vitali Fioletov, Pascal Hedelt, Diego Loyola, Thomas Wagner, Michel Van Roozendaël

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsEnvironment and Climate Change Canada
Fundersnot available
KeywordsSatelliteAlgorithmEnvironmental scienceChemistryComputer sciencePhysics

Abstract

fetched live from OpenAlex

Since nearly two years, the operational SO2 product from the TROPOspheric Monitoring Instrument (TROPOMI) onboard Sentinel-5 Precursor (S5P) platform has provided important information on volcanic and anthropogenic SO2 emissions, with an unprecedented level of details. In this presentation, we critically discuss the advantages and disadvantages of the current operational algorithm in light of the validation results obtained so far, and present how the retrieval scheme could evolve in the future. In the first part, we briefly present the main algorithm features and an overview of the SO2 product validation. One challenge in this respect is the current lack of ground-based SO2 measurements for anthropogenic source regions. We therefore rely largely on comparisons with other satellite datasets (e.g., OMI and OMPS). The main lesson learnt is that satellite SO2 retrievals generally agree very well for large SO2 columns (mostly volcanic) while persisting differences exist for low columns when different algorithms are compared. This motivates the second part of the presentation which aims at extensively comparing the results from existing S5P SO2 operational and scientific algorithms, notably DOAS and PCA retrievals (or other alternative approaches). Here, all configuration settings and auxiliary data (e.g. absorption cross-sections) are aligned in order to better understand the differences through sensitivity tests. This effort is not only important to improve the TROPOMI SO2 results but it is also particularly relevant in the context of the forthcoming Sentinel-4 mission that will mainly probe weak anthropogenic SO2 sources. The last part of the presentation gives a general overview of new features planned for the next versions of the operational SO2 algorithm.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.005
metaresearch head score (Gemma)0.008
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Methods · Consensus signal: none
Teacher disagreement score0.015
Threshold uncertainty score0.031

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0050.008
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0020.002
Open science0.0020.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0020.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.242
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2020
Admission routes1
Has abstractyes

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