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Record W3092206027 · doi:10.1107/s205322962001308x

Platinum(II) complex with 4-nitro-<i>N</i>-(pyridin-2-ylmethylidene)aniline: synthesis, characterization, crystal structure and antioxidant activity

2020· article· en· W3092206027 on OpenAlexaff
Mehdi Khalaj, Abolfazl Olyaei, Mahdieh Sadeghpour, Arash Lalegani, Janusz Lipkowski, Alan J. Lough

Bibliographic record

VenueActa Crystallographica Section C Structural Chemistry · 2020
Typearticle
Languageen
FieldMedicine
TopicMetal complexes synthesis and properties
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsSchiff baseDenticityChemistryAnilineCrystal structureAcetonitrileLigand (biochemistry)MoleculePlatinumNitroMedicinal chemistryHydrogen bondCrystallographyStereochemistryOrganic chemistryCatalysisAlkyl

Abstract

fetched live from OpenAlex

A novel complex has been prepared using the ( E )-4-nitro- N -(pyridin-2-ylmethylidene)aniline bidentate Schiff base ligand and PtCl 2 , namely, dichlorido[( E )-4-nitro- N -(pyridin-2-ylmethylidene)aniline-κ 2 N , N ′]platinum(II) acetonitrile hemisolvate, [PtCl 2 (C 12 H 9 N 3 O 2 )]·0.5CH 3 CN, 1 . According to the X-ray measurements of the crystal structure, the Pt II ion adopts a PtCl 2 N 2 square-planar coordination. The coordination of the Schiff base ligand to the Pt II ion occurs in a cyclic bidentate fashion, as a result of which a five-membered metallacycle is formed. Furthermore, in the structure of 1 , the neutral molecules form a one-dimensional chain structure through C—H...Cl and C—H...O hydrogen bonds. The characterization of the complex was performed via single-crystal X-ray diffraction, IR spectroscopy and elemental analysis, and the antioxidant activity of the complex was evaluated using spectrophotometry by the 1,1-diphenyl-2-picrylhydrazyl (DPPH) method.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.378
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.226
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

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Same venueActa Crystallographica Section C Structural ChemistrySame topicMetal complexes synthesis and propertiesFrench-language works237,207