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Record W3093175747 · doi:10.1063/5.0018016

Charge transport anisotropy in hot extruded bismuth telluride: Scattering by acoustic phonons

2020· article· en· W3093175747 on OpenAlexafffund
R. A. Masut, Cédric André, D. Vasilevskiy, S. Turenne

Bibliographic record

VenueJournal of Applied Physics · 2020
Typearticle
Languageen
FieldMaterials Science
TopicAdvanced Thermoelectric Materials and Devices
Canadian institutionsPolytechnique MontréalRegroupement Québécois sur les Matériaux de Pointe
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsCondensed matter physicsSeebeck coefficientThermoelectric effectMaterials scienceScatteringAnisotropyPhonon scatteringBismuth telluridePhononIsotropyThermoelectric materialsAtmospheric temperature rangeCharge carrierThermal conductivityComposite materialOpticsPhysicsThermodynamics

Abstract

fetched live from OpenAlex

A model of the thermoelectric transport properties of hot extruded bulk polycrystalline (HEBP) n-type Bi2Te3 has been developed based on the marked anisotropy of its properties induced by extrusion. HEBP Bi2Te3 is a highly textured material that allows treating electrical and thermal transport in the plane perpendicular to the extrusion axis as approximately isotropic. The model of this transport is based on the simplified electronic density of states suggested by ab initio calculations of the band structure of crystalline Bi2Te3 near the band edges. The proposed model can also be applied to transport along the extrusion axis in a temperature range when there is only one limiting charge carrier scattering mechanism. It provides excellent accord to the Hall effect (perpendicular) and the Harman (along extrusion) measurement of mobility, and the Seebeck coefficient of HEBP n-type Bi2Te3 in the temperature range from ∼200 to 460 K. It can be concluded that acoustic phonon scattering provides the limiting scattering mechanism for this temperature range. The model is also applied to elucidate the important role of thermodiffusion, suggesting that the usual approach to experimentally obtain this contribution to the thermal conductivity can only give approximate rough estimates.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.018
Threshold uncertainty score0.667

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.229
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2020
Admission routes2
Has abstractyes

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