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Record W3094147855 · doi:10.1063/5.0026040

Anisotropic, meandering domain microstructure in the improper ferroelectric CsNbW2O9

2020· article· en· W3094147855 on OpenAlexfundno aff
Shane J. McCartan, Patrick W. Turner, Jason A. McNulty, Jesi R. Maguire, Conor J. McCluskey, Finlay D. Morrison, J. M. Gregg, Ian MacLaren

Bibliographic record

VenueAPL Materials · 2020
Typearticle
Languageen
FieldMaterials Science
TopicMultiferroics and related materials
Canadian institutionsnot available
FundersQueen's UniversityQueen's University BelfastUniversity of GlasgowEngineering and Physical Sciences Research CouncilUniversity of St Andrews
KeywordsMicrostructureMaterials scienceFerroelectricityCondensed matter physicsDomain (mathematical analysis)Piezoresponse force microscopyManganiteAnisotropyDomain wall (magnetism)CrystallographyOpticsPhysicsComposite materialDielectricFerromagnetismChemistry

Abstract

fetched live from OpenAlex

The improper ferroelectric CsNbW2O9 has recently been highlighted as the first material outside the manganite family to exhibit a similar meandering, sixfold domain structure to that responsible for enhanced and diminished conduction at charged domain walls in the rare earth manganites. While there is no current evidence for variation in domain wall conduction relative to bulk in CsNbW2O9, the similarities in microstructure strongly suggest that charged domain walls are present in this material. Herein, we report a comprehensive study of the domain microstructure of CsNbW2O9 by both piezoresponse force microscopy and transmission electron microscopy to reveal that there are, in fact, clear distinctions in the domain structure of the two systems. Constraints arising from the crystal structure of CsNbW2O9, namely, the connectivity of the BO6 polyhedra and atomic displacements occurring purely along the c axis, mean that domain walls preferentially run parallel to the c direction (the polar axis of the material) and thus remain uncharged. The characteristic cloverleaf domain structure reminiscent of the manganites is still present; however, the structure meanders predominantly in the ab plane and, therefore, appears differently depending on the projection direction from which it is viewed. As a result of this microstructural constraint, charged domain walls are not prevalent in this material.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.228
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2020
Admission routes1
Has abstractyes

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