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Record W3097729847 · doi:10.1002/admt.202000704

Nanomechanical Gas Sensing with Laser Treated 2D Nanomaterials

2020· article· en· W3097729847 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Materials Technologies · 2020
Typearticle
Languageen
FieldEngineering
TopicGas Sensing Nanomaterials and Sensors
Canadian institutionsNational Institute for NanotechnologyUniversity of Waterloo
FundersJapan Society for the Promotion of ScienceNatural Sciences and Engineering Research Council of Canada
KeywordsGrapheneMaterials scienceNanomaterialsOxideMolybdenum disulfideNanotechnologyDopantBoron nitrideAdsorptionTungsten disulfideSurface modificationDopingChemical engineeringOptoelectronicsChemistryOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Abstract 2D nanomaterials such as graphene oxide (GO), molybdenum disulfide (MoS 2 ), and tungsten disulfide (WS 2 ) are viable candidates for use in chemical gas sensors due to their large specific surface area available for analyte adsorption. In this work, these 2D materials are treated with a femtosecond laser process to intentionally introduce defects, dopants, and functional groups to the material for improved gas adsorption properties. The materials are coated onto a nanomechanical membrane‐type surface stress sensor (MSS) to evaluate their sensing capability toward a select group of volatile organic compounds. By utilizing the MSS platform, the approach avoids the need for 2D materials with conductive properties typically required in chemoresistive sensors. The results show that a longer laser treatment time for graphene oxide increases the sensor response, which is attributed to an increase in defects and oxygen functional groups. Doping of graphene oxide with boron nitride improves sensor response, likely due to the introduction of pyrrolic nitrogen groups with high chemical activity. Additionally, the graphene oxides demonstrate partial selectivity toward the detection of toluene, attributable to π–π interactions. MoS 2 and WS 2 nanoflakes also show enhanced sensor response attributed to the formation of apical/bridging sulfur bonds with high catalytic activity.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.015
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.186
Teacher spread0.177 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it