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Time Delay in Molecular Photoionization

2017· article· en· W3104019560 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueFigshare · 2017
Typearticle
Languageen
FieldPhysics and Astronomy
TopicLaser-Matter Interactions and Applications
Canadian institutionsNational Research Council Canada
Fundersnot available
KeywordsPhotoionizationHomonuclear moleculeIonizationDiatomic moleculeAtomic physicsScatteringValence (chemistry)MoleculeChemistryMolecular physicsPhysicsIonQuantum mechanics

Abstract

fetched live from OpenAlex

Manuscript &amp; supplementary materials (.pdf), interactive figures (.fig) and data (.dat).<br>Update 30th June 2017: Added .dat files for full complex dipoles (N2 only).<br><br>Update 12th Feb 2017: Added PDF "Response to Comment on ``Time delays in molecular photoionization'': Extended Discussion &amp; Technical Notes". This is the technical response to a recent comment on the original article (to be published in J. Phys. B). Arxiv 1612.00481.Interested readers can also consult https://doi.org/10.6084/m9.figshare.c.3511731 for further background materials.<br>Update 11th July 2016: Added .dat files for Tw data (finally).<br>Update 1st June 2016: updated arxiv version of the manuscript. The published version can be found in J. Phys. B 49, 095602 (2016), doi: 10.1088/0953-4075/49/9/095602 (see link below).<br>Update 5th April 2016: added some additional notes on scattering theory &amp; use of ePolyScat.<br>Update 9th Feb. 2016: angular line-outs added to Supplementary Material PDF.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.775
Threshold uncertainty score0.993

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.2320.007

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.272
Teacher spread0.258 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it