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Record W3109199625 · doi:10.1002/cjce.23971

Full‐field <scp>PIV</scp> / <scp>DIA</scp> and local concentration measurements of ozone decomposition in riser‐flow

2020· article· en· W3109199625 on OpenAlexvenueno aff
Álvaro E. Carlos Varas, E.A.J.F. Peters, J.A.M. Kuipers

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2020
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsnot available
FundersNederlandse Organisatie voor Wetenschappelijk Onderzoek
KeywordsDecompositionFlow (mathematics)OzoneParticle (ecology)Mass transferMaterials scienceVolumetric flow rateMechanicsWork (physics)ChemistryThermodynamicsChromatographyPhysicsGeologyOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract A full‐field PIV‐DIA technique has been coupled to concentration measurements in order to characterize the riser performance at different gas superficial velocities and reaction rates for ozone decomposition. Experiments under riser flow conditions were performed with the use of a compact pseudo‐2D lab‐scale riser reactor. The purpose of this work is to generate reliable experimental data to validate computational models for mass transfer in riser flow conditions. The catalytic activity of the particles was characterized. To analyze the reaction rate effect over the performance of a riser reactor, two catalyst batches with different activities were used and their kinetics were measured. The hydrodynamics of the gas‐solid flow was determined using the PIV‐DIA technique. Particle clusters were identified and characterized. By correlating the cluster information and mass concentration measurements, it was shown that a higher frequency of local flow heterogeneities near the walls led to higher conversion rates than in the core of the riser. Reaction rate and gas superficial effects are analyzed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.217
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2020
Admission routes1
Has abstractyes

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Same venueThe Canadian Journal of Chemical EngineeringSame topicCatalytic Processes in Materials ScienceFrench-language works237,207