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Record W3115149690 · doi:10.1021/acsestwater.0c00183

Effects of Oil Sands Process-Affected Water on Measured Concentrations of Polycyclic Aromatic Hydrocarbons

2020· article· en· W3115149690 on OpenAlexafffund
Hattan A. Alharbi, Steve Wiseman, John P. Giesy

Bibliographic record

VenueACS ES&T Water · 2020
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of SaskatchewanUniversity of Lethbridge
FundersKing Saud UniversityNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsSyncrude
KeywordsChemistryEnvironmental chemistryAqueous solutionBioavailabilityAqueous two-phase systemOil sandsEnvironmental remediationFraction (chemistry)ContaminationChromatographyOrganic chemistryAsphalt

Abstract

fetched live from OpenAlex

The assessment of risks and remediation of oil sands process-affected water (OSPW) requires an understanding of possible interactions of naturally occurring surfactants with hydrophobic organic compounds, such as polycyclic aromatic hydrocarbons (PAHs). In this study, effects of the extractable organic fraction of OSPW (OF-OSPW) on rates of release and freely dissolved aqueous concentration of several PAHs were investigated using a passive dosing approach, in which a poly(dimethylsiloxane) (PDMS) film was loaded with PAHs of interest. The concentrations of PAHs released from PDMS into aqueous solutions were directly proportional to concentrations of OF-OSPW. PAHs reached equilibrium partitioning 1–4 h faster when the aqueous phase was OF-OSPW than when it was freshwater. Greater concentrations of PAHs were released from PDMS when OF-OSPW was reconstituted in saline water compared to when it was reconstituted in freshwater. Apparent aqueous solubilities of PAHs were greater in intact OSPW than in OF-OSPW. Measured concentrations of PAHs in various aqueous solutions of OSPW and salts correlated with log K ow of PAHs. This might be because of disruption of PAHs sorbed into PDMS. These results suggest that the bioavailability of PAHs can be greater in the presence of more polar organic compounds in OSPW.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.220
Teacher spread0.212 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2020
Admission routes2
Has abstractyes

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Same venueACS ES&T WaterSame topicPetroleum Processing and AnalysisFrench-language works237,207