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Record W3115723692

Effects of Formaldehyde on DNA: A Molecular Dynamics Study of Formaldehyde Adducts

2018· article· en· W3115723692 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueURSCA Proceedings · 2018
Typearticle
Languageen
FieldEnvironmental Science
TopicIndoor Air Quality and Microbial Exposure
Canadian institutionsUniversity of Lethbridge
Fundersnot available
KeywordsNucleobaseChemistryGuanineMoietyDNAAdductMolecular Structure of Nucleic Acids: A Structure for Deoxyribose Nucleic AcidHydrogen bondMolecular dynamicsStereochemistryDNA adductDNA damageFormaldehydeStackingBiochemistryBase pairComputational chemistryMoleculeOrganic chemistryNucleotideGene
DOInot available

Abstract

fetched live from OpenAlex

Formaldehyde is a known carcinogen, which damages and mutates DNA in the cells of mammals. Acute and chronic exposure to formaldehyde may occur in both occupational settings (e.g., embalmers) and from several household products (e.g., insulation, particle boards, and carpeting). Upon human exposure to formaldehyde, several DNA adducts may be formed, including those with the amino groups of guanine (denoted CH2OH-N2-G), cytosine (CH2OH-N4-C), and adenine (CH2OH-N6-A). Each of these adducts consists of a methoxy moiety linked to the exocyclic amino group of the respective DNA nucleobase. The methoxy moiety can interfere with several noncovalent interactions within a DNA helix, including Watson-Crick hydrogen bonding, Hoogsteen hydrogen bonding, and stacking interactions between neighboring DNA nucleobases. These interactions are essential to the normal function of DNA and their disruption could lead to mutations when DNA is copied, which in turn lead to health effects such as cancer. Although insight into the implications on formaldehyde adducts are currently lacking from experimental studies, computational chemistry can be used to predict the effects of the methoxy moiety on the nucleobase interactions and the mutagenicity of these adducts. In the current study, molecular dynamics (MD) simulations, along with advanced structural analysis and energy calculations, were used to study the preferred conformations of the nucleobase within damaged DNA, and thereby characterize the structural impacts of this damage. Using this analysis, key insight was gained into the mutagenicity of the CH2OH adducts and the data obtained can be used to direct future biochemical studies of the harmful effects of these lesions. *Indicates presenter

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.048
Threshold uncertainty score0.775

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.212
Teacher spread0.207 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it