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Record W3118279471 · doi:10.1038/s41535-020-00302-5

Nematic fluctuations in iron-oxychalcogenide Mott insulators

2021· article· en· W3118279471 on OpenAlexaff
Byron Freelon, Rajib Sarkar, Sirko Kamusella, F. Brückner, Vadim Grinenko, Swagata Acharya, M. S. Laad, L. Craco, Z. Yamani, Roxana Flacau, I. P. Swainson, Benjamin A. Frandsen, R. J. Birgeneau, Yuhao Liu, Bhupendra Karki, Alaa Alfailakawi, Jöerg C. Neuefeind, Michelle Everett, Hangdong Wang, Binjie Xu, Minghu Fang, H.‐H. Klauß

Bibliographic record

Venuenpj Quantum Materials · 2021
Typearticle
Languageen
FieldMaterials Science
TopicIron-based superconductors research
Canadian institutionsCanadian Nuclear Laboratories
FundersLawrence Berkeley National LaboratoryFundamental Research Funds for the Central UniversitiesOffice of ScienceCoordenação de Aperfeiçoamento de Pessoal de Nível SuperiorOak Ridge National LaboratoryConselho Nacional de Desenvolvimento Científico e TecnológicoNational Natural Science Foundation of ChinaBasic Energy SciencesUT-BattelleBattelleZhejiang UniversityDeutsche ForschungsgemeinschaftU.S. Department of Energy
KeywordsCondensed matter physicsLiquid crystalPhysicsSuperconductivityAnisotropyCuprateSpin (aerodynamics)MagnetismNeutron diffractionQuantum mechanicsDiffraction

Abstract

fetched live from OpenAlex

Abstract Nematic fluctuations occur in a wide range physical systems from biological molecules to cuprates and iron pnictide high- T c superconductors. It is unclear whether nematicity in pnictides arises from electronic spin or orbital degrees of freedom. We studied the iron-based Mott insulators La 2 O 2 Fe 2 OM 2 M = (S, Se), which are structurally similar to pnictides. Nuclear magnetic resonance revealed a critical slowing down of nematic fluctuations and complementary Mössbauerr spectroscopy data showed a change of electrical field gradient. The neutron pair distribution function technique detected local C 2 fluctuations while neutron diffraction indicates that global C 4 symmetry is preserved. A geometrically frustrated Heisenberg model with biquadratic and single-ion anisotropic terms provides the interpretation of the low temperature magnetic fluctuations. The nematicity is not due to spontaneous orbital order, instead it is linked to geometrically frustrated magnetism based on orbital selectivity. This study highlights the interplay between orbital order and spin fluctuations in nematicity.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0200.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.298
Teacher spread0.270 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2021
Admission routes1
Has abstractyes

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