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Record W3120301037 · doi:10.1016/j.jhazmat.2021.125130

A cross scale investigation of galena oxidation and controls on mobilization of lead in mine waste rock

2021· article· en· W3120301037 on OpenAlexafffund
Zhongwen Bao, Tom A. Al, Martin Couillard, Glenn Poirier, Jeff Bain, Heather K. Shrimpton, Y. Zou Finfrock, Antonio Lanzirotti, Doğan Paktunç, Emily M. Saurette, Yongfeng Hu, Carol J. Ptacek, David W. Blowes

Bibliographic record

VenueJournal of Hazardous Materials · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicMine drainage and remediation techniques
Canadian institutionsNatural Resources CanadaCanadian Light Source (Canada)National Research Council CanadaUniversity of WaterlooCanadian Museum of NatureWilfrid Laurier UniversityUniversity of Ottawa
FundersArgonne National LaboratoryNatural Sciences and Engineering Research Council of CanadaCanadian Institutes of Health ResearchOffice of ScienceCanadian Light SourceCrown-Indigenous Relations and Northern Affairs CanadaU.S. Department of EnergyUniversity of ChicagoNational Science Foundation
KeywordsGalenaCovelliteDissolutionEnvironmental chemistryChemistryCarbonateWeatheringMineralogySulfidePore water pressureGeologyGeochemistryPyriteSphaleriteOrganic chemistryChalcopyriteGeotechnical engineering

Abstract

fetched live from OpenAlex

to the surficial environment and commonly causes the formation of anglesite (in acidic environments) or cerussite (in alkaline environments). However, conditions prevalent in weathering environments are diverse and different reaction mechanisms reflect this variability at various scales. Here we applied complementary techniques across a range of scales, from nanometers to 10 s of meters, to study the oxidation of galena and accumulation of secondary phases that influence the release and mobilization of Pb within a sulfide-bearing waste-rock pile. Within the neutral-pH pore-water environment, the oxidation of galena releases Pb ions resulting in the formation of secondary Pb-bearing carbonate precipitates. Cerussite is the dominant phase and shannonite is a possible minor phase. Dissolved Cu from the pore water reacts at the surface of galena, forming covellite at the interface. Nanometer scale characterization suggests that secondary covellite is intergrown with secondary Pb-bearing carbonates at the interface. A small amount of the S derived from galena is sequestered with the secondary covellite, but the majority of the S is oxidized to sulfate and released to the pore water.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.031
Threshold uncertainty score0.223

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.244
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations45
Published2021
Admission routes2
Has abstractyes

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