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Record W3120390283 · doi:10.1016/j.ecmx.2020.100074

Recovery approaches for sulfuric acid from the concentrated acid hydrolysis of lignocellulosic feedstocks: A mini-review

2021· article· en· W3120390283 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueEnergy Conversion and Management X · 2021
Typearticle
Languageen
FieldEngineering
TopicBiofuel production and bioconversion
Canadian institutionsUniversité de Sherbrooke
FundersMitacs
KeywordsSulfuric acidChemistryLignocellulosic biomassHydrolysisHydrolysateSugarChromatographyExtraction (chemistry)Ion chromatographyBiomass (ecology)Pulp and paper industryOrganic chemistry

Abstract

fetched live from OpenAlex

The two-step concentrated acid hydrolysis approach is a very efficient method for the generation of monomeric sugars from lignocellulosic biomass, due to its ability to generate near-theoretical sugar yields, at moderate processing times. Sulfuric acid is the most frequently employed acid due to its combination of low cost, high efficiency, and low toxicity and corrosivity compared to other acids. A challenge with this approach is the ability to recover and re-use the acid catalyst in order to make the process economical and reduce waste streams. This paper reviews different acid recovery techniques found in literature and compare them based on performance. The three most investigated and best performing approaches are ion exclusion chromatography, solvent extraction and electrodialysis. Of these, ion exclusion chromatography is the most investigated, and also applied at bigger scale for recovering acid from the final sugar hydrolysate stream. Solvent extraction is a popular option when acid recovery is performed on the intermediate product stream in the two-step process. The studied techniques achieve high acid recovery performance and acid-sugar separation efficiencies, with acid recoveries of 90–99% reported, with low loss of sugars (higher than 90% glucose yields). More research is required into the impact on process performance of re-using the acid catalyst after recovery.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.659
Threshold uncertainty score0.479

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.185
Teacher spread0.167 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it