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Record W3126549621 · doi:10.5194/amt-14-945-2021

Quantifying fugitive gas emissions from an oil sands tailings pond with open-path Fourier transform infrared measurements

2021· article· en· W3126549621 on OpenAlexafffundabout
Yuan You, Samar G. Moussa, Lucas Zhang, Long Fu, James N. Beck, Ralf M. Staebler

Bibliographic record

VenueAtmospheric measurement techniques · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsSuncor Energy (Canada)Alberta Environment and Protected AreasEnvironment and Climate Change Canada
FundersAlbert Einstein College of Medicine, Yeshiva UniversityNatural Resources CanadaEnvironment and Climate Change CanadaSuncor Energy Incorporated
KeywordsEddy covarianceFugitive emissionsFlux (metallurgy)Environmental scienceMethaneOil sandsAtmospheric sciencesDispersion (optics)Atmosphere (unit)TailingsGreenhouse gasEnvironmental chemistrySoil scienceChemistryMeteorologyGeologyMaterials sciencePhysicsEcosystem

Abstract

fetched live from OpenAlex

Fugitive emissions from tailings ponds contribute significantly to facility emissions in the Alberta oil sands, but details on chemical emission profiles and the temporal and spatial variability of emissions to the atmosphere are sparse, since flux measurement techniques applied for compliance monitoring have their limitations. In this study, open-path Fourier transform infrared spectroscopy was evaluated as a potential alternative method for quantifying spatially representative fluxes for various pollutants (methane, ammonia, and alkanes) from a particular pond, using vertical-flux-gradient and inverse-dispersion methods. Gradient fluxes of methane averaged 4.3 g m −2 d −1 but were 44 % lower than nearby eddy covariance measurements, while inverse-dispersion fluxes agreed to within 30 %. With the gradient fluxes method, significant NH 3 emission fluxes were observed (0.05 g m −2 d −1 , 42 t yr −1 ), and total alkane fluxes were estimated to be 1.05 g m −2 d −1 (881 t yr −1 ), representing 9.6 % of the facility emissions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.078
Threshold uncertainty score0.155

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.264
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations19
Published2021
Admission routes3
Has abstractyes

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