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Record W3127334261 · doi:10.1002/cjce.24009

Improving the accuracy of the Eyring equation by pseudo‐ideal solution model to predict the viscosity of the mono‐ethanol amine‐[Bmim] <scp>PF6</scp> ionic liquid blends in a <scp>CO<sub>2</sub></scp> capturing pilot plant

2021· article· en· W3127334261 on OpenAlexvenueno aff
Hamid Reza Kalatjari, Mohammad Reza Jafari Nasr, Ali Haghtalab, Amir Heydarinasab

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2021
Typearticle
Languageen
FieldChemical Engineering
TopicIonic liquids properties and applications
Canadian institutionsnot available
Fundersnot available
KeywordsIonic liquidViscositySolventElectrolyteThermodynamicsAmine gas treatingRelative viscosityActivation energyChemistryMaterials scienceChemical engineeringOrganic chemistryPhysical chemistryPhysics

Abstract

fetched live from OpenAlex

Abstract The purpose of the present study was to propose a new simulation model for calculation of the viscosity of the mono‐ethanol amine‐ionic liquid (MEA‐IL) solvent in the CO2‐capturing pilot plant. To do so, a combination of the pseudo‐ideal solution model (PISM) and Eyring's mixture viscosity equation was implemented in MATLAB. Moreover, the various thermodynamic models were used to calculate viscosity, using solvent containing MEA‐IL in the high CO2 feed gas. The present study determined the viscosities of the MEA‐IL blends at different concentrations and various temperatures in the CO2 capturing pilot plant. The results were comparable to those obtained from the Eyring‐PISM model, Eyring‐Wilson method, Cheng and Meisen a previous study equation, and the Aspen Plus and Promax with electrolyte non‐random two‐liquid model that presented the actual viscosity values of the liquid solutions. The calculated solvent viscosity values with the Eyring‐PISM model at different temperature profiles were achieved using an average absolute deviation (AAD) of about 1.164% and 1.422% in absorber and desorber for solvent (MEA = 27 wt% and IL = 34.2 wt%) and 1.578% and 1.868% in absorber and desorber for solvent (MEA = 29 wt% and IL = 37.12 wt%), respectively. The consideration of a suitable model for the determination of viscosity has a significant role in energy consumption in the CO2‐capturing pilot plant. The estimated energy consumption with the Eyring‐PISM model was achieved using an AAD of about 0.652% for solvent (MEA = 27 wt% and IL = 34.2 wt%) and 0.502% for solvent (MEA = 29 wt% and IL = 37.12 wt%), respectively. The results obtained from the Eyring‐PISM simulation model using the experimental data revealed a high degree of accuracy.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.007
Threshold uncertainty score0.015

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.197
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations1
Published2021
Admission routes1
Has abstractyes

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