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Record W3127409601 · doi:10.1103/physrevb.103.054107

Machine learning metadynamics simulation of reconstructive phase transition

2021· article· en· W3127409601 on OpenAlexafffund
Qunchao Tong, Xiaoshan Luo, Adebayo A. Adeleke, Pengyue Gao, Yu Xie, Hanyu Liu, Quan Li, Yanchao Wang, Jian Lv, Yansun Yao, Yanming Ma

Bibliographic record

VenuePhysical review. B./Physical review. B · 2021
Typearticle
Languageen
FieldMaterials Science
TopicMachine Learning in Materials Science
Canadian institutionsUniversity of Saskatchewan
FundersProgram for Jilin University Science and Technology Innovative Research TeamFundamental Research Funds for the Central UniversitiesNational Key Research and Development Program of ChinaChina Postdoctoral Science FoundationNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of China
KeywordsMetadynamicsPhase transitionMolecular dynamicsComputer scienceStatistical physicsEmbedded atom modelDensity functional theoryScalingRepresentation (politics)Computational scienceAlgorithmPhysicsMathematicsThermodynamicsQuantum mechanicsGeometry

Abstract

fetched live from OpenAlex

Simulating reconstructive phase transition requires an accurate description of potential energy surface (PES). Density-functional-theory (DFT) based molecular dynamics can achieve the desired accuracy but it is computationally unfeasible for large systems and/or long simulation times. Here we introduce an approach that combines the metadynamics simulation and machine learning representation of PES at the accuracy close to the DFT calculations, but with the computational cost several orders of magnitude less, and scaling with system size approximately linear. The high accuracy of the method is demonstrated in the simulation of pressure-induced $B4\text{\ensuremath{-}}B1$ phase transition in gallium nitride (GaN). The large-scale simulation using a 4096-atom simulation box reveals the phase transition with excellent detail, revealing different simulated transition paths under particular stress conditions. With well-trained machine learning potentials, this method can be easily applied to all types of systems for accurate scalable simulations of solid-solid reconstructive phase transition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.392
Teacher spread0.373 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations27
Published2021
Admission routes2
Has abstractyes

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Same venuePhysical review. B./Physical review. BSame topicMachine Learning in Materials ScienceFrench-language works237,207